Asymmetric Vacancies Efficiently Couple O <sub>2</sub> Activation With Reactive Oxygen Species Evolution for Enhanced Photocatalytic Methane Conversion
delivers the highest turnover number (TON) reported to date among Ag-based catalysts for the photocatalytic oxidative coupling of methane via a ROS-mediated pathway. The general effectiveness of this asymmetric-vacancy strategy is further validated in other representative photocatalytic reactions, including hydrogen peroxide production and the oxidative coupling of benzyl alcohol.
Authors
- Qh Zhang
- Shunji Xie (ORCID: https://orcid.org/0000-0002-5324-8638)
- S Y Wang
- Xuejiao Wu (ORCID: https://orcid.org/0000-0002-1116-6060)
- Huizhen Zhang (ORCID: https://orcid.org/0000-0001-7253-9740)
- Ye Wang (ORCID: https://orcid.org/0000-0003-0764-2279)
- Haoyang Liu
Institutions
- Collaborative Innovation Center of Chemistry for Energy Materials (CN)
- Fuzhou University (CN)
Publication Details
- Journal
- Angewandte Chemie International Edition
- Published
- 2026-04-20
- DOI
- https://doi.org/10.1002/anie.7358043
- Primary Topic
- Advanced Photocatalysis Techniques
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Natural Science Foundation of China
- Natural Science Foundation of Fujian Province
- Fundamental Research Funds for the Central Universities