Frequency Stability of Graphene Nonlinear Parametric Oscillator

High-frequency stability is crucial for the performance of graphene resonators in sensing and timekeeping applications. However, the extreme miniaturization and high mechanical compliance that make graphene attractive also render it highly susceptible to nonlinearities, degrading frequency stability. Here, we demonstrate that graphene parametric oscillators provide an alternative nonlinear operating regime, where short-term frequency stability can be enhanced despite strong nonlinearity. By operating graphene resonators in a phase-locked loop, we experimentally demonstrate that parametric oscillations in the postbifurcation regime achieve lower Allan deviation at fast integration times than Duffing oscillations at identical amplitudes. This improvement originates from strong nonlinear damping inherent to parametric oscillators, which suppresses amplitude-to-frequency noise conversion at large amplitudes. A minimal theoretical model captures observed phase diffusion and identifies nonlinear damping as the dominant mechanism governing phase noise reduction. These results highlight the role of nonlinear dissipation in enabling precision sensing beyond conventional limits of graphene oscillators.

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Publication Details

Journal
Nano Letters
Published
2026-04-21
DOI
https://doi.org/10.1021/acs.nanolett.6c00581
Primary Topic
Mechanical and Optical Resonators
Type
article
Field-Weighted Citation Impact
0.00

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article

Frequency Stability of Graphene Nonlinear Parametric Oscillator

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Frequency Stability of Graphene Nonlinear Parametric Oscillator

Oriel Shoshani, Tomás Manzaneque, Alberto Martín-Pérez, Farbod Alijani, Enise Kartal, Elena Botnaru
article en

Abstract

High-frequency stability is crucial for the performance of graphene resonators in sensing and timekeeping applications. However, the extreme miniaturization and high mechanical compliance that make graphene attractive also render it highly susceptible to nonlinearities, degrading frequency stability. Here, we demonstrate that graphene parametric oscillators provide an alternative nonlinear operating regime, where short-term frequency stability can be enhanced despite strong nonlinearity. By operating graphene resonators in a phase-locked loop, we experimentally demonstrate that parametric oscillations in the postbifurcation regime achieve lower Allan deviation at fast integration times than Duffing oscillations at identical amplitudes. This improvement originates from strong nonlinear damping inherent to parametric oscillators, which suppresses amplitude-to-frequency noise conversion at large amplitudes. A minimal theoretical model captures observed phase diffusion and identifies nonlinear damping as the dominant mechanism governing phase noise reduction. These results highlight the role of nonlinear dissipation in enabling precision sensing beyond conventional limits of graphene oscillators.

Nano Letters
Ben-Gurion University of the Negev (IL), Delft University of Technology (NL)
Israel Science Foundation, Ben-Gurion University of the Negev, European Research Council
Openalex Percentile: Top 6%
Mechanical and Optical Resonators
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