Selective Reversible Hydrolysis at Inequivalent Oxygen Sites Driven by Framework Al in MFI Zeolites Revealed by <sup>17</sup> O NMR Spectroscopy and DFT Calculations

O-based probing strategy offers an efficient approach to elucidate reversible hydrolysis at inequivalent oxygen sites, contributing to the rational design of hydrothermally stable zeolites.

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Publication Details

Journal
Journal of the American Chemical Society
Published
2026-04-17
DOI
https://doi.org/10.1021/jacs.6c00010
Primary Topic
Zeolite Catalysis and Synthesis
Type
article
Field-Weighted Citation Impact
0.00

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article

Selective Reversible Hydrolysis at Inequivalent Oxygen Sites Driven by Framework Al in MFI Zeolites Revealed by 17 O NMR Spectroscopy and DFT Calculations

J F Sun, Fuxiang Zhang, Feng‐Shou Xiao, Yingxu Wei et al.
Journal of the American Chemical Society
Zeolite Catalysis and Synthesis
article

Selective Reversible Hydrolysis at Inequivalent Oxygen Sites Driven by Framework Al in MFI Zeolites Revealed by 17 O NMR Spectroscopy and DFT Calculations

J F Sun, Fuxiang Zhang, Feng‐Shou Xiao, Yingxu Wei, Caiyi Lou, Shutao Xu, Liang Wang, Jing Niu, C ZHANG, Junjie Li, Wenna Zhang, Yanan Zhang, Linhai He, Zhongmin Liu
article en

Abstract

O-based probing strategy offers an efficient approach to elucidate reversible hydrolysis at inequivalent oxygen sites, contributing to the rational design of hydrothermally stable zeolites.

Journal of the American Chemical SocietyVol. 148(17)
Ministry of Education (NZ), Dalian Institute of Chemical Physics (CN), Chinese Academy of Sciences (CN), Dalian National Laboratory for Clean Energy (CN), University of Chinese Academy of Sciences (CN), Zhejiang University (CN)
National Natural Science Foundation of China
Openalex Percentile: Top 27%
Zeolite Catalysis and Synthesis
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