Vortex Stability and Magnetic Disorder Tolerance in Magnetic High-Entropy Alloy Superconductor NbTaTiZrNi

High-entropy alloy (HEA) superconductors offer mechanical robustness and tunable compositions. We report the synthesis and characterization of a Ni-containing HEA, NbTaTiZrNi, which exhibits superconductivity with Tc ≈ 7.1 K and weak itinerant ferromagnetism up to 300 K, with coercive fields Hcoer ≈ 100–300 Oe. While magnetic elements often suppress superconductivity via pair breaking, Tc in this Ni-containing alloy remains comparable to nonmagnetic Ta1/6Nb2/6Ti1/6Zr1/6Hf1/6 (Tc ≈ 7.8 K). Thermomagnetic flux avalanches are not observed, and critical current densities reach 104–105 A cm–2 at 2 K, indicating robust vortex stability in this composition. Electrical resistivity, magnetization, and specific-heat measurements indicate conventional s-wave superconductivity with intermediate electron–phonon coupling (λ ≈ 0.7). The observed vortex-pinning behavior is consistent with a mixed landscape of grain-boundary and point-like defects, likely influenced by configurational disorder and Ni distribution, though Fe-rich secondary phases may also contribute. These results demonstrate that this specific Ni-containing HEA exhibits robust superconductivity with flux-stable behavior, providing a platform for further exploration of high-performance superconductors in cryogenic applications.

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Publication Details

Journal
ACS Applied Electronic Materials
Published
2026-04-17
DOI
https://doi.org/10.1021/acsaelm.6c00009
Primary Topic
High Entropy Alloys Studies
Type
article
Field-Weighted Citation Impact
0.00

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article

Vortex Stability and Magnetic Disorder Tolerance in Magnetic High-Entropy Alloy Superconductor NbTaTiZrNi

Heon‐Jung Kim, Rahmatul Hidayati, Beongki Cho, Jong‐Soo Rhyee et al.
ACS Applied Electronic Materials
High Entropy Alloys Studies
article

Vortex Stability and Magnetic Disorder Tolerance in Magnetic High-Entropy Alloy Superconductor NbTaTiZrNi

Heon‐Jung Kim, Rahmatul Hidayati, Beongki Cho, Jong‐Soo Rhyee, Kwan‐Young Lee, Jin Hee Kim, Jae Hyun Yun, Dilanath Adhikari
article en

Abstract

High-entropy alloy (HEA) superconductors offer mechanical robustness and tunable compositions. We report the synthesis and characterization of a Ni-containing HEA, NbTaTiZrNi, which exhibits superconductivity with Tc ≈ 7.1 K and weak itinerant ferromagnetism up to 300 K, with coercive fields Hcoer ≈ 100–300 Oe. While magnetic elements often suppress superconductivity via pair breaking, Tc in this Ni-containing alloy remains comparable to nonmagnetic Ta1/6Nb2/6Ti1/6Zr1/6Hf1/6 (Tc ≈ 7.8 K). Thermomagnetic flux avalanches are not observed, and critical current densities reach 104–105 A cm–2 at 2 K, indicating robust vortex stability in this composition. Electrical resistivity, magnetization, and specific-heat measurements indicate conventional s-wave superconductivity with intermediate electron–phonon coupling (λ ≈ 0.7). The observed vortex-pinning behavior is consistent with a mixed landscape of grain-boundary and point-like defects, likely influenced by configurational disorder and Ni distribution, though Fe-rich secondary phases may also contribute. These results demonstrate that this specific Ni-containing HEA exhibits robust superconductivity with flux-stable behavior, providing a platform for further exploration of high-performance superconductors in cryogenic applications.

ACS Applied Electronic MaterialsVol. 8(8)
King Fahd University of Petroleum and Minerals (SA), Kyung Hee University (KR), Gwangju Institute of Science and Technology (KR), Centre of Excellence for Advanced Materials (CN), Advanced Energy Materials (United States) (US), Graduate School USA (US), Daegu University (KR)
Ministry of Trade, Industry and Energy, National Research Foundation of Korea
Openalex Percentile: Top 17%
High Entropy Alloys Studies
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