Josephson Diode and Spin-valve Effects on the Surface of Altermagnet CrSb

We experimentally investigate charge transport in In-CrSb and In-CrSb-In proximity devices, which are formed as junctions between superconducting indium leads and thick single crystal flakes of altermagnet CrSb. For double In-CrSb-In junctions, dV / dI ( B ) curves are mirrored in respect to zero field for two magnetic field sweep directions, which is characteristic behavior of a Josephson spin valve. Also, we demonstrate Josephson diode effect by direct measurement of the critical current for two opposite directions in external magnetic field. We interpret these observations as a joint effect of the spin-polarized topological surface states and the altermagnetic spin splitting of the bulk bands in CrSb. For a single In-CrSb interface, the superconducting gap oscillates in magnetic field for both field orientations, which strongly resembles the Fulde–Ferrell–Larkin–Ovchinnikov (FFLO) behavior. FFLO is based on finite-momentum Cooper pairing, therefore, it is fully compatible with the requirements for the Josephson diode effect.