Disorder-Induced Griffiths-like Phase and Charge Localization in Sr <sub>2</sub> FeRuO <sub>6</sub>

A comprehensive understanding of complex transition-metal oxides is key to designing next-generation spintronic materials with tailored magnetic and transport functionalities. We investigate the interplay among structural disorder, frustrated magnetism, and localized charge transport in the 3d–4d hybrid double perovskite Sr2FeRuO6. The compound adopts a monoclinic structure with significant B-site antisite disorder that drives its unconventional behavior. Magnetic measurements uncover a robust Griffiths phase extending well above the ordering temperature, evidencing stable short-range ferromagnetic clusters within a disordered matrix. Electrical transport remains strongly localized, transitioning from small-polaron hopping at high temperatures to variable-range hopping at intermediate temperatures. These results position Sr2FeRuO6 as a representative 3d–4d hybrid system in which quenched disorder stabilizes spin inhomogeneity, while polaronic and hopping transport are also observed.

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Publication Details

Journal
The Journal of Physical Chemistry C
Published
2026-04-16
DOI
https://doi.org/10.1021/acs.jpcc.6c01836
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
0.00

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article

Disorder-Induced Griffiths-like Phase and Charge Localization in Sr 2 FeRuO 6

Shuvendu Ghosh, Koustav Pal, I. Das
The Journal of Physical Chemistry C
Advanced Condensed Matter Physics
article

Disorder-Induced Griffiths-like Phase and Charge Localization in Sr 2 FeRuO 6

Shuvendu Ghosh, Koustav Pal, I. Das
article en

Abstract

A comprehensive understanding of complex transition-metal oxides is key to designing next-generation spintronic materials with tailored magnetic and transport functionalities. We investigate the interplay among structural disorder, frustrated magnetism, and localized charge transport in the 3d–4d hybrid double perovskite Sr2FeRuO6. The compound adopts a monoclinic structure with significant B-site antisite disorder that drives its unconventional behavior. Magnetic measurements uncover a robust Griffiths phase extending well above the ordering temperature, evidencing stable short-range ferromagnetic clusters within a disordered matrix. Electrical transport remains strongly localized, transitioning from small-polaron hopping at high temperatures to variable-range hopping at intermediate temperatures. These results position Sr2FeRuO6 as a representative 3d–4d hybrid system in which quenched disorder stabilizes spin inhomogeneity, while polaronic and hopping transport are also observed.

The Journal of Physical Chemistry CVol. 130(17)
University of Engineering & Management (IN), Saha Institute of Nuclear Physics (IN), Homi Bhabha National Institute (IN), Integrated Optoelectronics (Norway) (NO), Institute of Environmental Studies & Wetland Management (IN), Aditya Birla (India) (IN), South China University of Technology (CN)
South China University of Technology, Saha Institute of Nuclear Physics, Department of Atomic Energy, Government of India
Openalex Percentile: Top 21%
Advanced Condensed Matter Physics
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