Investigating Effect of Decoherence on Fano Interference through Raman Spectroscopy
mode in p-type doped silicon is examined. The decoherence is demonstrated by introducing random phase fluctuation to the energy-dependent scattering phase Δ(ε) appearing in the typical Fano treatment with the help of a stochastic Monte Carlo approach, and a complete methodology is presented to explain the changes in the Raman line shape. Our approach successfully explains observed changes in the intensity and line shape of mode, suggesting that decoherence is a crucial factor controlling the Raman profiles.
Authors
- Omkar V. Rambadey (ORCID: https://orcid.org/0000-0001-8379-0965)
- Pankaj R. Sagdeo (ORCID: https://orcid.org/0000-0002-2475-6676)
- Nikita Jain
- Payal Ratnawat
Institutions
- Indian Institute of Technology Indore (IN)
Publication Details
- Journal
- The Journal of Physical Chemistry Letters
- Published
- 2026-04-16
- DOI
- https://doi.org/10.1021/acs.jpclett.6c00804
- Primary Topic
- Thermal properties of materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Department of Science and Technology, Ministry of Science and Technology, India
- Ministry of Education, India
- Indian Institute of Technology Indore
- Science and Engineering Research Board