Investigating Effect of Decoherence on Fano Interference through Raman Spectroscopy

mode in p-type doped silicon is examined. The decoherence is demonstrated by introducing random phase fluctuation to the energy-dependent scattering phase Δ(ε) appearing in the typical Fano treatment with the help of a stochastic Monte Carlo approach, and a complete methodology is presented to explain the changes in the Raman line shape. Our approach successfully explains observed changes in the intensity and line shape of mode, suggesting that decoherence is a crucial factor controlling the Raman profiles.

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Publication Details

Journal
The Journal of Physical Chemistry Letters
Published
2026-04-16
DOI
https://doi.org/10.1021/acs.jpclett.6c00804
Primary Topic
Thermal properties of materials
Type
article
Field-Weighted Citation Impact
0.00

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article

Investigating Effect of Decoherence on Fano Interference through Raman Spectroscopy

Omkar V. Rambadey, Pankaj R. Sagdeo, Nikita Jain, Payal Ratnawat
The Journal of Physical Chemistry Letters
Thermal properties of materials
article

Investigating Effect of Decoherence on Fano Interference through Raman Spectroscopy

Omkar V. Rambadey, Pankaj R. Sagdeo, Nikita Jain, Payal Ratnawat
article en

Abstract

mode in p-type doped silicon is examined. The decoherence is demonstrated by introducing random phase fluctuation to the energy-dependent scattering phase Δ(ε) appearing in the typical Fano treatment with the help of a stochastic Monte Carlo approach, and a complete methodology is presented to explain the changes in the Raman line shape. Our approach successfully explains observed changes in the intensity and line shape of mode, suggesting that decoherence is a crucial factor controlling the Raman profiles.

The Journal of Physical Chemistry LettersVol. 17(17)
Indian Institute of Technology Indore (IN)
Department of Science and Technology, Ministry of Science and Technology, India, Ministry of Education, India, Indian Institute of Technology Indore, Science and Engineering Research Board
Affordable and clean energy
Openalex Percentile: Top 26%
Thermal properties of materials
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