Mechano-Programmable Circularly Polarized Luminescent Elastomers for Dynamic Information Encryption and Chiral Logic Gates

-hydroxyethyl methacrylate) matrix. The resulting elastomer simultaneously achieves efficient mechanophore activation, a robust chiral environment, and excellent mechanical compatibility (breaking strength ≈ 18 MPa, breaking strain ≈ 450%). It exhibits force-dependent, in situ, continuous, and reversible CPL responses. By further incorporation of a benzothiadiazole (BTz) green fluorophore, multicolor CPL outputs spanning green, orange, and red are realized under a single mechanical stimulus. Leveraging this programmable multidimensional optical behavior, we demonstrate mechanically triggered dynamic information encryption with hierarchical authentication and multi-input chiral logic gates. This work establishes a versatile platform for next-generation intelligent anticounterfeiting materials with in situ, mechano-regulated, and multiband CPL capabilities.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2026-04-14
DOI
https://doi.org/10.1021/acsami.6c03348
Primary Topic
Luminescence and Fluorescent Materials
Type
article
Field-Weighted Citation Impact
0.00

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article

Mechano-Programmable Circularly Polarized Luminescent Elastomers for Dynamic Information Encryption and Chiral Logic Gates

Yifan Bai, Xiaoshuai Huang, Yuan Yuan, Bing-Hao Liu et al.
ACS Applied Materials & Interfaces
Luminescence and Fluorescent Materials
article

Mechano-Programmable Circularly Polarized Luminescent Elastomers for Dynamic Information Encryption and Chiral Logic Gates

Yifan Bai, Xiaoshuai Huang, Yuan Yuan, Bing-Hao Liu, Hui Wang, Shi-Yi Li
article en

Abstract

-hydroxyethyl methacrylate) matrix. The resulting elastomer simultaneously achieves efficient mechanophore activation, a robust chiral environment, and excellent mechanical compatibility (breaking strength ≈ 18 MPa, breaking strain ≈ 450%). It exhibits force-dependent, in situ, continuous, and reversible CPL responses. By further incorporation of a benzothiadiazole (BTz) green fluorophore, multicolor CPL outputs spanning green, orange, and red are realized under a single mechanical stimulus. Leveraging this programmable multidimensional optical behavior, we demonstrate mechanically triggered dynamic information encryption with hierarchical authentication and multi-input chiral logic gates. This work establishes a versatile platform for next-generation intelligent anticounterfeiting materials with in situ, mechano-regulated, and multiband CPL capabilities.

ACS Applied Materials & InterfacesVol. 18(16)
Tianjin University (CN), Jilin University (CN), Jilin Medical University (CN), State Key Laboratory of Supramolecular Structure and Materials
Natural Science Foundation of Jilin Province, National Natural Science Foundation of China
Openalex Percentile: Top 24%
Luminescence and Fluorescent Materials
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