Deprotonation-Induced Strong Covalent Interfacial Bonding Stabilizes the Solid Electrolyte Interphase and Raises the Performance of Lithium-Ion Batteries
, while maintaining the capacity retention of 81% over 300 and 78% over 600 cycles. The present work reveals the deprotonation-driven interphase stability mechanism and establishes active-component regulation as a new paradigm for high-energy density lithium-ion batteries.
Authors
- Fei Wang (ORCID: https://orcid.org/0000-0001-6890-619X)
- Francesco Ciucci (ORCID: https://orcid.org/0000-0003-0614-5537)
- Xingyang Wang (ORCID: https://orcid.org/0009-0005-1843-1268)
- Baptiste Py (ORCID: https://orcid.org/0000-0003-1294-6138)
- Lewis Kien Juen Ting (ORCID: https://orcid.org/0000-0002-2027-7635)
- Jingyuan Li (ORCID: https://orcid.org/0000-0001-9660-0542)
- Qing Wang (ORCID: https://orcid.org/0000-0002-0263-3579)
- Shengjun Xu
- Chengzhi Zhang
- Zhendong Liu
- Qi Zhao
- Yulin Gao
- Shuqi Wang
Institutions
- Shanghai University (CN)
- Chongqing University (CN)
- National University of Singapore (SG)
- Hong Kong University of Science and Technology (HK)
- Ji Hua Laboratory (CN)
- Fujian Research Institute of Light Industry (CN)
- ECSI Fibrotools (United States) (US)
- Institute of Refrigeration (GB)
- University of Bayreuth (DE)
- South China University of Technology (CN)
Publication Details
- Journal
- Journal of the American Chemical Society
- Published
- 2026-04-13
- DOI
- https://doi.org/10.1021/jacs.5c23319
- Primary Topic
- Advancements in Battery Materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Agency for Science, Technology and Research
- National Research Foundation Singapore
- National Natural Science Foundation of China