Mesoscopic Hydrophobic Microenvironment Engineering on a Single-Atom Catalyst for Steering CO <sub>2</sub> Photoreduction to CH <sub>4</sub>
, with notable activity preserved even under 700 nm irradiation. This work underscores that governing the mass transport of key intermediates at the mesoscale is a decisive design principle for steering catalytic selectivity.
Authors
- Yakun Qu (ORCID: https://orcid.org/0000-0002-2670-209X)
- Xiuyi Yang (ORCID: https://orcid.org/0000-0001-8892-2373)
- William Orbell
- Xiaoguang Zhao
- Bo Meng (ORCID: https://orcid.org/0009-0001-4628-0787)
- Haiwei Su
- Haibo Yin
- Yunlong Wang
- Junhua Li
- Feng Dong
- Jianjun Chen
- Zhen Chen
- Lin Chen
- Lin Guo
Institutions
- Sinopec (China) (CN)
- State Key Joint Laboratory of Environment Simulation and Pollution Control (CN)
- Beijing Advanced Sciences and Innovation Center (CN)
- Sinopec Research Institute of Petroleum Processing
- Beihang University (CN)
- Tsinghua University (CN)
Publication Details
- Journal
- Journal of the American Chemical Society
- Published
- 2026-04-06
- DOI
- https://doi.org/10.1021/jacs.6c01672
- Primary Topic
- CO2 Reduction Techniques and Catalysts
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Natural Science Foundation of China
- Tsinghua University
- China Petrochemical Corporation