Transient Deformation and Charge Evolution during Alternating Current-Electrohydrodynamic Oscillations of Confined Droplets

This study investigates the transient electrohydrodynamic behavior of a confined, neutrally buoyant droplet subjected to a cyclic electric field, focusing on the coupled evolution of interfacial charge, deformation, and flow. Both the droplet and the surrounding medium are modeled as Newtonian, immiscible leaky-dielectric fluids under creeping-flow and small-deformation conditions. Confinement is shown to significantly dampen droplet oscillations by enhancing viscous dissipation in thin fluid gaps, restricting internal and external circulation, and increasing hydrodynamic resistance that opposes electrically induced Maxwell stresses. The transient response is decomposed into mean and time-periodic components to examine two conductivity configurations, in which the droplet is either more or less conductive than the surrounding medium. The effects of confinement ratio, oscillation frequency, and electrical property contrasts are systematically analyzed to quantify their influence on deformation amplitude, flow-field strength, and interfacial stress balance. Increasing the confinement suppresses time-dependent deformation by limiting flow development and amplifying viscous resistance, leading to a marked reduction in oscillation amplitude. The role of the relaxation frequency in governing the electrical response is examined by distinguishing conduction- and displacement-dominated regimes. At low frequencies, rapid charge relaxation promotes strong interfacial charge accumulation and enhanced electrohydrodynamic forcing, resulting in pronounced deformation and circulation. At higher frequencies, displacement currents dominate, interfacial charge weakens, and both deformation and flow are attenuated, particularly under confinement. Phase lags between the applied electric field, interfacial charge, and electric fields inside and outside the droplet are quantified and shown to depend on confinement, fluid properties, and excitation frequency. The results provide physical insight into frequency-dependent electrohydrodynamic droplet dynamics in confined environments relevant to microfluidic and droplet-based technologies.

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Publication Details

Journal
Langmuir
Published
2026-04-03
DOI
https://doi.org/10.1021/acs.langmuir.6c00048
Citations
1
Primary Topic
Electrohydrodynamics and Fluid Dynamics
Type
article
Field-Weighted Citation Impact
13.00

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article

Transient Deformation and Charge Evolution during Alternating Current-Electrohydrodynamic Oscillations of Confined Droplets

Pulak Gupta, Devranjan Samanta, Purbarun Dhar
1 citations
Langmuir
Electrohydrodynamics and Fluid Dynamics
13.00
article

Transient Deformation and Charge Evolution during Alternating Current-Electrohydrodynamic Oscillations of Confined Droplets

Pulak Gupta, Devranjan Samanta, Purbarun Dhar
article en
1 citations

Abstract

This study investigates the transient electrohydrodynamic behavior of a confined, neutrally buoyant droplet subjected to a cyclic electric field, focusing on the coupled evolution of interfacial charge, deformation, and flow. Both the droplet and the surrounding medium are modeled as Newtonian, immiscible leaky-dielectric fluids under creeping-flow and small-deformation conditions. Confinement is shown to significantly dampen droplet oscillations by enhancing viscous dissipation in thin fluid gaps, restricting internal and external circulation, and increasing hydrodynamic resistance that opposes electrically induced Maxwell stresses. The transient response is decomposed into mean and time-periodic components to examine two conductivity configurations, in which the droplet is either more or less conductive than the surrounding medium. The effects of confinement ratio, oscillation frequency, and electrical property contrasts are systematically analyzed to quantify their influence on deformation amplitude, flow-field strength, and interfacial stress balance. Increasing the confinement suppresses time-dependent deformation by limiting flow development and amplifying viscous resistance, leading to a marked reduction in oscillation amplitude. The role of the relaxation frequency in governing the electrical response is examined by distinguishing conduction- and displacement-dominated regimes. At low frequencies, rapid charge relaxation promotes strong interfacial charge accumulation and enhanced electrohydrodynamic forcing, resulting in pronounced deformation and circulation. At higher frequencies, displacement currents dominate, interfacial charge weakens, and both deformation and flow are attenuated, particularly under confinement. Phase lags between the applied electric field, interfacial charge, and electric fields inside and outside the droplet are quantified and shown to depend on confinement, fluid properties, and excitation frequency. The results provide physical insight into frequency-dependent electrohydrodynamic droplet dynamics in confined environments relevant to microfluidic and droplet-based technologies.

LangmuirVol. 42(14)
Indian Institute of Technology Ropar (IN), Indian Institute of Technology Kharagpur (IN), Czech Academy of Sciences, Institute of Hydrology (CZ)
National Natural Science Foundation of China, Natural Science Foundation of Guangdong Province, State Key Laboratory of Luminescent Materials and Devices, National Science and Technology Major Project, National Key Research and Development Program of China
Openalex Percentile: Top 1%
Electrohydrodynamics and Fluid Dynamics
13.00
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