Deterministic Integration of CsPbBr <sub>3</sub> Quantum Dots with Plasmonic Ring Microcavities

Perovskite quantum dots hold great promise for quantum information processing as wavelength-tunable single photon sources operable over a broad temperature range. However, their deterministic integration into nanophotonic structures remains a major challenge limited by their random spatial distribution and nondirectional emission. In this work, we employ a two-step electron beam lithography process to deterministically place CsPbBr3 quantum dots within the mode volume of plasmonic ring microcavities. Simulations predict strong field enhancement within the cavity, boosting photon emission rates via the Purcell effect and improving the quantum efficiency of the emitters. Experimentally, coupling ensembles of CsPbBr3 quantum dots to the cavities results in a 4-fold enhancement in photoluminescence intensity and a 3-fold reduction in photoluminescence lifetime at room temperature. Single-emitter coupling is further investigated at cryogenic temperatures, leading to a 2-fold reduction in photoluminescence lifetime. These results demonstrate a potentially scalable approach for the integration of perovskite quantum dots into nanophotonic cavities and quantum photonic circuits.

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Publication Details

Journal
ACS Photonics
Published
2026-04-01
DOI
https://doi.org/10.1021/acsphotonics.5c01863
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
0.00

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article

Deterministic Integration of CsPbBr 3 Quantum Dots with Plasmonic Ring Microcavities

Jingzhong Yang, Pengji Li, Chenxi Ma, Gabriele Rainò et al.
ACS Photonics
Strong Light-Matter Interactions
article

Deterministic Integration of CsPbBr 3 Quantum Dots with Plasmonic Ring Microcavities

Jingzhong Yang, Pengji Li, Chenxi Ma, Gabriele Rainò, Yeşim Müge Şahin, Maximilian Heller, Eddy P. Rugeramigabo, Franziska Krieg, Michael Zopf, Tom N. Rakow, Xian Zheng, Fei Ding, Johann Dzeik, Maksym V. Kovalenko
article en

Abstract

Perovskite quantum dots hold great promise for quantum information processing as wavelength-tunable single photon sources operable over a broad temperature range. However, their deterministic integration into nanophotonic structures remains a major challenge limited by their random spatial distribution and nondirectional emission. In this work, we employ a two-step electron beam lithography process to deterministically place CsPbBr3 quantum dots within the mode volume of plasmonic ring microcavities. Simulations predict strong field enhancement within the cavity, boosting photon emission rates via the Purcell effect and improving the quantum efficiency of the emitters. Experimentally, coupling ensembles of CsPbBr3 quantum dots to the cavities results in a 4-fold enhancement in photoluminescence intensity and a 3-fold reduction in photoluminescence lifetime at room temperature. Single-emitter coupling is further investigated at cryogenic temperatures, leading to a 2-fold reduction in photoluminescence lifetime. These results demonstrate a potentially scalable approach for the integration of perovskite quantum dots into nanophotonic cavities and quantum photonic circuits.

ACS PhotonicsVol. 13(8)
Leibniz University Hannover (DE), ETH Zurich (CH), Institute of Inorganic Chemistry of the Slovak Academy of Sciences (SK), Applied Thin Films (United States) (US), Swiss Federal Laboratories for Materials Science and Technology (CH)
Deutsche Forschungsgemeinschaft, Bundesministerium für Bildung und Forschung, China Scholarship Council, Niedersächsisches Ministerium für Wissenschaft und Kultur
Affordable and clean energy
Openalex Percentile: Top 23%
Strong Light-Matter Interactions
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