Multicarrier electrical and thermal magnetotransport in altermagnetic CrSb

Chromium antimonide has emerged as a key material platform for studying altermagnetism because of its simple binary composition, high Néel temperature, and semimetallic electronic structure. Here, we investigate electrical and thermal magnetotransport in single-crystalline CrSb using steady- and pulsed-magnetic fields up to 65 T, and complement these measurements with neutron diffraction and magnetization data. We confirm the compensated magnetic structure and observe a large nonsaturating magnetoresistance together with a pronounced nonlinear Hall response at low temperatures. Multicarrier modeling, supported by mobility-spectrum analysis, reveals coexisting electron- and holelike charge carriers with mobilities up to ∼ 3000 cm 2 / Vs and shows that the number of transport channels that can be resolved strongly depends on the accessible magnetic-field range. Thermal-transport measurements further reveal a nonlinear thermal Hall response and a thermal conductivity substantially exceeding a simple Wiedemann-Franz law. The broadly similar field and temperature evolution of electrical and thermal transport point to a dominant electronic contribution, while the remaining deviations indicate additional heat-carrying channels.

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Publication Details

Journal
Physical Review Materials
Published
2026-10-13
DOI
https://doi.org/10.1103/xn7y-df6x
Citations
1
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
2.76

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Multicarrier electrical and thermal magnetotransport in altermagnetic CrSb

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Physical Review Materials
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article

Multicarrier electrical and thermal magnetotransport in altermagnetic CrSb

Markéta Žáčková, Marein C. Rahn, Helena Reichlová, Srikanta Goswami, Tommy Kotte, Michał Baj, Reza Firouzmandi, M. Uhlarz, Jiří Pospíšil, Antonín Baďura, Fabio Orlandi, Philipp Ritzinger, Th. Speliotis, Dominik Kriegner, Sven Luther, Vilmos Kocsis, Toni Helm, Jochen Wosnitza, Sajal Naduvile Thadathil, Dr Pascal Manuel, Václav Petříček, Lorenz Farin, Christoph Müller, Bernd Büchner
article en
1 citations

Abstract

Chromium antimonide has emerged as a key material platform for studying altermagnetism because of its simple binary composition, high Néel temperature, and semimetallic electronic structure. Here, we investigate electrical and thermal magnetotransport in single-crystalline CrSb using steady- and pulsed-magnetic fields up to 65 T, and complement these measurements with neutron diffraction and magnetization data. We confirm the compensated magnetic structure and observe a large nonsaturating magnetoresistance together with a pronounced nonlinear Hall response at low temperatures. Multicarrier modeling, supported by mobility-spectrum analysis, reveals coexisting electron- and holelike charge carriers with mobilities up to ∼ 3000 cm 2 / Vs and shows that the number of transport channels that can be resolved strongly depends on the accessible magnetic-field range. Thermal-transport measurements further reveal a nonlinear thermal Hall response and a thermal conductivity substantially exceeding a simple Wiedemann-Franz law. The broadly similar field and temperature evolution of electrical and thermal transport point to a dominant electronic contribution, while the remaining deviations indicate additional heat-carrying channels.

Physical Review MaterialsVol. 10(10)
Czech Academy of Sciences (CZ), Charles University (CZ), Helmholtz-Zentrum Dresden-Rossendorf (DE), Leibniz Institute for Solid State and Materials Research (DE), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), ISIS Neutron and Muon Source, University of Warsaw (PL), Technische Universität Dresden (DE)
UK Research and Innovation, European Commission, Deutsche Forschungsgemeinschaft, Ministerstvo Školství, Mládeže a Tělovýchovy, Grantová Agentura České Republiky, Max-Planck-Gesellschaft, Akademie Věd České Republiky, Science and Technology Facilities Council, Staatssekretariat für Bildung, Forschung und Innovation
Openalex Percentile: Top 12%
Magnetic properties of thin films
2.76
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