Cementitious Mortars as Structural Supercapacitors: Role of Zeolite Additives and Moisture Evolution

This study aims to investigate the potential for using commercial building materials such as cement and quarry sand for developing functional building components with electrical energy storage capacities. Cubic specimens of cement mortars made from commercial Portland cement and quarry sand were fabricated, while commercial galvanized mesh, used for mortar reinforcement, was used as electrodes. Moreover, natural zeolites were used as additives to modify mortar electrical properties. Cyclic voltammetry (CV), and electrochemical impedance spectroscopy (EIS) were used to assess the capacity of the fabricated specimens for electrical energy storage. Results indicated that the studied cement mortars modified with natural zeolites behave as a non-ideal electrical double-layer capacitor (EDLC) with stable capacitive behavior over time. This makes these cementitious materials promising for further research in electrical energy storage applications.