Sustained poling-induced second-order optical nonlinearity in sodium-doped amorphous niobium oxide waveguides

Nonlinear optical devices have attracted increasing interest, with lithium niobate being the benchmark material due to its strong second-order optical nonlinearity (SONL). However, its hardness, chemical inertness, and anisotropy present significant fabrication challenges, motivating the search for alternative platforms. Amorphous materials with poling-induced SONL offer promising opportunities, as their isotropic nature enables flexible optical design. In this work, we investigate amorphous sodium niobate thin films and demonstrate waveguide structures with active SONL through thermally controlled micrometer-scale poling combined with standard lithography. Using polarized second-harmonic generation (SHG) microscopy, we show precise spatial and geometrical control of the induced SONL, and its retention after waveguide processing steps, including UV lithography and dry-etching. The persistence of strong SHG signals, particularly near poling electrode edges, highlights the potential of aligning lithography mask with SONL patterns to enhance device performance, providing a foundation for developing efficient nonlinear photonic devices based on poled amorphous thin films.

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Journal
Scientific Reports
Published
2026-03-26
DOI
https://doi.org/10.1038/s41598-026-45779-5
Primary Topic
Photorefractive and Nonlinear Optics
Type
article
Field-Weighted Citation Impact
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article

Sustained poling-induced second-order optical nonlinearity in sodium-doped amorphous niobium oxide waveguides

Lara Karam, Miloš Nedeljković, Sirawit Boonsit, Ganapathy Senthil Murugan et al.
Scientific Reports
Photorefractive and Nonlinear Optics
article

Sustained poling-induced second-order optical nonlinearity in sodium-doped amorphous niobium oxide waveguides

Lara Karam, Miloš Nedeljković, Sirawit Boonsit, Ganapathy Senthil Murugan, Lydie Bourgeois, Frederic Adamietz, Nadege Courjal, Marc Dussauze
article en

Abstract

Nonlinear optical devices have attracted increasing interest, with lithium niobate being the benchmark material due to its strong second-order optical nonlinearity (SONL). However, its hardness, chemical inertness, and anisotropy present significant fabrication challenges, motivating the search for alternative platforms. Amorphous materials with poling-induced SONL offer promising opportunities, as their isotropic nature enables flexible optical design. In this work, we investigate amorphous sodium niobate thin films and demonstrate waveguide structures with active SONL through thermally controlled micrometer-scale poling combined with standard lithography. Using polarized second-harmonic generation (SHG) microscopy, we show precise spatial and geometrical control of the induced SONL, and its retention after waveguide processing steps, including UV lithography and dry-etching. The persistence of strong SHG signals, particularly near poling electrode edges, highlights the potential of aligning lithography mask with SONL patterns to enhance device performance, providing a foundation for developing efficient nonlinear photonic devices based on poled amorphous thin films.

Scientific Reports
Université de Bordeaux (FR), Franche-Comté Électronique Mécanique Thermique et Optique - Sciences et Technologies (FR), Institut des Sciences Moléculaires (FR), University of Southampton (GB)
Industry, innovation and infrastructure
Openalex Percentile: Top 6%
Photorefractive and Nonlinear Optics
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Sustained poling-induced second-order optical nonlinearity in sodium-doped amorphous niobium oxide waveguides — Lara Karam, Miloš Nedeljković, et al. · Scientific Reports (2026) | TGRS Research Map | TGRS