Laser direct writing and Raman Stokes contrast screening of quantum emitter sites in hBN
Laser direct writing (LDW) enables the spatially defined creation of room-temperature single-photon emitters (SPEs) in hexagonal boron nitride (hBN). However, the rapid characterization of written sites remains a bottleneck, and the available toolset for efficient screening is limited. Here, we demonstrate a streamlined LDW workflow utilizing single-shot pulses combined with a confocal screening technique that exploits the hBN E<sub>2g</sub> Stokes line to rapidly localize and map laser-modified regions without relying a priori on defect photoluminescence (PL). This approach enables the direct correlation of site morphology with PL hotspots, revealing that the emergence of single-photon emitters coincides with a threshold regime of minimal lattice modification. Micro-Raman spectral mapping further uncovers localized compressive strain surrounding these emission sites. We classify the generated defects into two families: narrowband "red" emitters (650-750 nm) with weak phonon sidebands (PSB), and 600-650 nm emitters with stronger vibronic coupling, both exhibiting linear polarization and high single-photon purity. These results establish a practical protocol for rapid prototyping, offering a valuable addition to the characterization toolkit for scalable quantum nanophotonics.
Authors
- Danielis Rutkauskas (ORCID: https://orcid.org/0000-0003-4705-2222)
- Tadas Paulauskas (ORCID: https://orcid.org/0000-0003-3776-0452)
- Edgaras Markauskas (ORCID: https://orcid.org/0000-0002-4304-8720)
- Martynas Talaikis (ORCID: https://orcid.org/0000-0003-3516-6425)
- Virginijus Bukauskas (ORCID: https://orcid.org/0000-0003-0275-9603)
- J. Janušonis
- Skirmantas Keršulis (ORCID: https://orcid.org/0000-0002-1815-357X)
- Viktorija Nargelienė (ORCID: https://orcid.org/0000-0001-7798-590X)
- Vakaris Šilys
- Ifra Bibi
Institutions
- Center for Physical Sciences and Technology (LT)
Publication Details
- Journal
- Discover Nano
- Published
- 2026-03-26
- DOI
- https://doi.org/10.1186/s11671-026-04530-9
- Primary Topic
- Diamond and Carbon-based Materials Research
- Type
- article
- Field-Weighted Citation Impact
- 0.00