Laser direct writing and Raman Stokes contrast screening of quantum emitter sites in hBN

Laser direct writing (LDW) enables the spatially defined creation of room-temperature single-photon emitters (SPEs) in hexagonal boron nitride (hBN). However, the rapid characterization of written sites remains a bottleneck, and the available toolset for efficient screening is limited. Here, we demonstrate a streamlined LDW workflow utilizing single-shot pulses combined with a confocal screening technique that exploits the hBN E<sub>2g</sub>​ Stokes line to rapidly localize and map laser-modified regions without relying a priori on defect photoluminescence (PL). This approach enables the direct correlation of site morphology with PL hotspots, revealing that the emergence of single-photon emitters coincides with a threshold regime of minimal lattice modification. Micro-Raman spectral mapping further uncovers localized compressive strain surrounding these emission sites. We classify the generated defects into two families: narrowband "red" emitters (650-750 nm) with weak phonon sidebands (PSB), and 600-650 nm emitters with stronger vibronic coupling, both exhibiting linear polarization and high single-photon purity. These results establish a practical protocol for rapid prototyping, offering a valuable addition to the characterization toolkit for scalable quantum nanophotonics.

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Publication Details

Journal
Discover Nano
Published
2026-03-26
DOI
https://doi.org/10.1186/s11671-026-04530-9
Primary Topic
Diamond and Carbon-based Materials Research
Type
article
Field-Weighted Citation Impact
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article

Laser direct writing and Raman Stokes contrast screening of quantum emitter sites in hBN

Danielis Rutkauskas, Tadas Paulauskas, Edgaras Markauskas, Martynas Talaikis et al.
Discover Nano
Diamond and Carbon-based Materials Research
article

Laser direct writing and Raman Stokes contrast screening of quantum emitter sites in hBN

Danielis Rutkauskas, Tadas Paulauskas, Edgaras Markauskas, Martynas Talaikis, Virginijus Bukauskas, J. Janušonis, Skirmantas Keršulis, Viktorija Nargelienė, Vakaris Šilys, Ifra Bibi
article en

Abstract

Laser direct writing (LDW) enables the spatially defined creation of room-temperature single-photon emitters (SPEs) in hexagonal boron nitride (hBN). However, the rapid characterization of written sites remains a bottleneck, and the available toolset for efficient screening is limited. Here, we demonstrate a streamlined LDW workflow utilizing single-shot pulses combined with a confocal screening technique that exploits the hBN E<sub>2g</sub>​ Stokes line to rapidly localize and map laser-modified regions without relying a priori on defect photoluminescence (PL). This approach enables the direct correlation of site morphology with PL hotspots, revealing that the emergence of single-photon emitters coincides with a threshold regime of minimal lattice modification. Micro-Raman spectral mapping further uncovers localized compressive strain surrounding these emission sites. We classify the generated defects into two families: narrowband "red" emitters (650-750 nm) with weak phonon sidebands (PSB), and 600-650 nm emitters with stronger vibronic coupling, both exhibiting linear polarization and high single-photon purity. These results establish a practical protocol for rapid prototyping, offering a valuable addition to the characterization toolkit for scalable quantum nanophotonics.

Discover NanoVol. 21(1)
Center for Physical Sciences and Technology (LT)
Quality Education
Openalex Percentile: Top 8%
Diamond and Carbon-based Materials Research
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