Strain-Engineered Deterministic Quantum Dots for Telecom O-Band Emission Using Buried Stressors

Abstract The deterministic realization of quantum light sources operating at telecom wavelengths is essential for long-distance fiber-based quantum communication and distributed quantum computing. In this work, we demonstrate that telecom O-band emission can be achieved from site-controlled InGaAs/GaAs quantum dots (QDs). Our concept utilizes a buried AlAs/AlOx stressor layer with the unique feature of inducing a well-defined and controllable tensile strain field at the growth surface, enabling both site-selective nucleation at the mesa’s centers and a redshift of QD emission to the ∼1.3 μm wavelength range. This concept not only eliminates the need for strain-reducing layers (SRLs), which are known to degrade optical coherence, but also provides spatial control and spectral tunability. The grown telecom QDs show single-photon emission with g(2)(0) = (5.0 ± 1.0) × 10–2 at 4 K and (2.8 ± 0.3) × 10–1 at 77 K, demonstrating the quantum nature and thermal stability of the emitters. The emission characteristics of complex excitonic states are analyzed using 8-band k·p and configuration-interaction modeling, which quantitatively reproduces the experimental observations. Finally, we present a theory-supported strategy to further redshift the emission toward the center of the O-band and beyond by employing a multiburied stressor approach. This combined framework of experiment and theory establishes the buried stressor concept as a scalable route toward highly coherent, position-controlled O-band quantum emitters compatible with scalable photonic integration.

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Publication Details

Journal
ACS Nano
Published
2026-10-26
DOI
https://doi.org/10.1021/acsnano.6c07558
Primary Topic
Semiconductor Quantum Structures and Devices
Type
article
Field-Weighted Citation Impact
0.00

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article

Strain-Engineered Deterministic Quantum Dots for Telecom O-Band Emission Using Buried Stressors

Ching‐Wen Shih, Sarthak Tripathi, Imad Limame, Kartik Gaur et al.
5 links
ACS Nano
Semiconductor Quantum Structures and Devices
article

Strain-Engineered Deterministic Quantum Dots for Telecom O-Band Emission Using Buried Stressors

Ching‐Wen Shih, Sarthak Tripathi, Imad Limame, Kartik Gaur, Sven Rodt, Petr Klenovský, Maximilian Ries, Martin Podhorský, Aris Koulas‐Simos, Stephan Reitzenstein, Setthanat Wijitpatima, Chirag C. Palekar, Dominik M. Feder
article en

Abstract

Abstract The deterministic realization of quantum light sources operating at telecom wavelengths is essential for long-distance fiber-based quantum communication and distributed quantum computing. In this work, we demonstrate that telecom O-band emission can be achieved from site-controlled InGaAs/GaAs quantum dots (QDs). Our concept utilizes a buried AlAs/AlOx stressor layer with the unique feature of inducing a well-defined and controllable tensile strain field at the growth surface, enabling both site-selective nucleation at the mesa’s centers and a redshift of QD emission to the ∼1.3 μm wavelength range. This concept not only eliminates the need for strain-reducing layers (SRLs), which are known to degrade optical coherence, but also provides spatial control and spectral tunability. The grown telecom QDs show single-photon emission with g(2)(0) = (5.0 ± 1.0) × 10–2 at 4 K and (2.8 ± 0.3) × 10–1 at 77 K, demonstrating the quantum nature and thermal stability of the emitters. The emission characteristics of complex excitonic states are analyzed using 8-band k·p and configuration-interaction modeling, which quantitatively reproduces the experimental observations. Finally, we present a theory-supported strategy to further redshift the emission toward the center of the O-band and beyond by employing a multiburied stressor approach. This combined framework of experiment and theory establishes the buried stressor concept as a scalable route toward highly coherent, position-controlled O-band quantum emitters compatible with scalable photonic integration.

ACS Nano
Masaryk University (CZ), Český metrologický institut (CZ), Thermo Fisher Scientific (Germany) (DE), Technische Universität Berlin (DE)
Volkswagen Foundation, Bundesministerium für Bildung und Forschung, HORIZON EUROPE European Innovation Council
Openalex Percentile: Top 80%
Semiconductor Quantum Structures and Devices
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