Impact of higher-order exchange on the lifetime of skyrmions and antiskyrmions

Abstract Reliable control of skyrmion lifetime is essential for realizing spintronic devices, yet the role of higher-order exchange—which can lead to skyrmion stabilization—remains largely unexplored. Here we calculate lifetimes of isolated skyrmions and antiskyrmions at transition-metal interfaces based on an atomistic spin model that includes all fourth-order exchange terms. Within harmonic transition-state theory, we evaluate both energetic and entropic contributions and find substantially enhanced lifetimes when higher-order exchange is included. The four-spin four-site interaction raises the energy barrier and lowers the curvature of the energy landscape at the collapse saddle point, increasing the pre-exponential factor. We show that skyrmions and antiskyrmions can remain thermally stable even without Dzyaloshinskii-Moriya interaction (DMI), and that tuning the four-spin term by a small amount modulates the prefactor over orders of magnitude. Our results identify higher-order exchange as a promising route to stabilize topological magnetic textures—in particular in systems lacking DMI—and to engineer their thermally activated decay.

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Publication Details

Journal
npj Computational Materials
Published
2026-03-23
DOI
https://doi.org/10.1038/s41524-026-02034-9
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
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article

Impact of higher-order exchange on the lifetime of skyrmions and antiskyrmions

Moritz A. Goerzen, Soumyajyoti Haldar, Stefan Heinze, Pavel F. Bessarab et al.
npj Computational Materials
Magnetic properties of thin films
article

Impact of higher-order exchange on the lifetime of skyrmions and antiskyrmions

Moritz A. Goerzen, Soumyajyoti Haldar, Stefan Heinze, Pavel F. Bessarab, Bjarne Beyer, Hendrik Schrautzer
article en

Abstract

Abstract Reliable control of skyrmion lifetime is essential for realizing spintronic devices, yet the role of higher-order exchange—which can lead to skyrmion stabilization—remains largely unexplored. Here we calculate lifetimes of isolated skyrmions and antiskyrmions at transition-metal interfaces based on an atomistic spin model that includes all fourth-order exchange terms. Within harmonic transition-state theory, we evaluate both energetic and entropic contributions and find substantially enhanced lifetimes when higher-order exchange is included. The four-spin four-site interaction raises the energy barrier and lowers the curvature of the energy landscape at the collapse saddle point, increasing the pre-exponential factor. We show that skyrmions and antiskyrmions can remain thermally stable even without Dzyaloshinskii-Moriya interaction (DMI), and that tuning the four-spin term by a small amount modulates the prefactor over orders of magnitude. Our results identify higher-order exchange as a promising route to stabilize topological magnetic textures—in particular in systems lacking DMI—and to engineer their thermally activated decay.

npj Computational MaterialsVol. 12(1)
Centre National de la Recherche Scientifique (FR), University of Iceland (IS), Université Fédérale de Toulouse Midi-Pyrénées (FR), Linnaeus University (SE), Christian-Albrechts-Universität zu Kiel (DE), Centre d’Élaboration de Matériaux et d’Études Structurales (FR)
Affordable and clean energy
Openalex Percentile: Top 11%
Magnetic properties of thin films
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