Highly Stable Chip-Scale Tellurium Memtransistor Based on Field-Induced Oxygen Vacancy Migration

Memtransistors have recently attracted attention as promising synaptic devices owing to their precise conductance tunability and heterosynaptic functionality, which can enhance the energy efficiency and integration density of neuromorphic systems. However, previous memtransistors have had difficulty controlling the lateral resistive switching characteristics and reproducibility to achieve a high yield and electrical durability. In this study, highly stable chip-scale Te memtransistor switching based on Schottky barrier height modulation from field-induced oxygen vacancy migration in TeO<sub>2-<i>x</i></sub> was demonstrated. The thickness of the radiofrequency (RF)-sputtered polycrystalline Te is a critical parameter in modulating the resistive behavior with gating tunability because the percentage of TeO<sub>2-<i>x</i></sub> in the Te film can be precisely controlled by its thickness. The Te memtransistor device can emulate heterosynaptic plasticity through voltage stimuli to the drain and gate terminals. The statistical distribution of the synaptic plasticity indicated that 62 devices were functional across an 8 × 8 memtransistor array in a single chip, providing a high yield of >96.9%. Additionally, the device exhibited high linearity and low asymmetry during potentiation/depression endurance cycling over 10 000 pulses. Furthermore, high pattern-recognition accuracy (∼94.2%) for handwritten numbers in a simulation task validated this promising method for the synaptic components of neuromorphic circuits. This study contributes significantly to the design diversity and large-scale integration of neuromorphic systems.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2026-03-16
DOI
https://doi.org/10.1021/acsami.5c20005
Primary Topic
Transition Metal Oxide Nanomaterials
Type
article
Field-Weighted Citation Impact
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article

Highly Stable Chip-Scale Tellurium Memtransistor Based on Field-Induced Oxygen Vacancy Migration

Y.S. Kim, Eunjeong Cho, S. K. OH, Wondeok Seo et al.
ACS Applied Materials & Interfaces
Transition Metal Oxide Nanomaterials
article

Highly Stable Chip-Scale Tellurium Memtransistor Based on Field-Induced Oxygen Vacancy Migration

Y.S. Kim, Eunjeong Cho, S. K. OH, Wondeok Seo, W. Park, Yong-Il Kwon, Min Jeong Kim, Jongwon YOON, Shinhoi Kim, Ojun Kwon, Minhee Kim, Yedam Kim, Byungjin Cho
article en

Abstract

Memtransistors have recently attracted attention as promising synaptic devices owing to their precise conductance tunability and heterosynaptic functionality, which can enhance the energy efficiency and integration density of neuromorphic systems. However, previous memtransistors have had difficulty controlling the lateral resistive switching characteristics and reproducibility to achieve a high yield and electrical durability. In this study, highly stable chip-scale Te memtransistor switching based on Schottky barrier height modulation from field-induced oxygen vacancy migration in TeO<sub>2-<i>x</i></sub> was demonstrated. The thickness of the radiofrequency (RF)-sputtered polycrystalline Te is a critical parameter in modulating the resistive behavior with gating tunability because the percentage of TeO<sub>2-<i>x</i></sub> in the Te film can be precisely controlled by its thickness. The Te memtransistor device can emulate heterosynaptic plasticity through voltage stimuli to the drain and gate terminals. The statistical distribution of the synaptic plasticity indicated that 62 devices were functional across an 8 × 8 memtransistor array in a single chip, providing a high yield of >96.9%. Additionally, the device exhibited high linearity and low asymmetry during potentiation/depression endurance cycling over 10 000 pulses. Furthermore, high pattern-recognition accuracy (∼94.2%) for handwritten numbers in a simulation task validated this promising method for the synaptic components of neuromorphic circuits. This study contributes significantly to the design diversity and large-scale integration of neuromorphic systems.

ACS Applied Materials & Interfaces
Chungbuk National University (KR), Korea Institute of Materials Science (KR), Chungbuk National University Hospital (KR)
Openalex Percentile: Top 20%
Transition Metal Oxide Nanomaterials
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