Aesthetic Profiling and Exploratory Composting Screening of Wood-Fiber Biocomposites Bonded with Spent Coffee Grounds and Ammonium Lignosulfonate
Spent coffee grounds (SCGs) and lignin-derived binders, such as ammonium lignosulfonate (ALS), are increasingly being explored as renewable resources to reduce reliance on conventional formaldehyde-based resins in wood-fiber biocomposites. Although prior work has shown that SCG-ALS adhesive systems can achieve promising mechanical performance, two practical aspects essential for industrial applications and circular design remain insufficiently explored: a predictable and reproducible visual appearance and credible end-of-life options. In this study, sustainable wood-fiber biocomposites bonded with SCG and ALS were assessed from an aesthetic performance and end-of-life perspective. Color was quantified in the CIE L*a*b* (CIELAB) space and expressed as total color difference (ΔE*) relative to a reference panel. Increasing total SCG + ALS content from 40 to 75 wt.% based on oven-dry fibers produced pronounced darkening, with lightness decreasing from L* = 47.1 to 34.3 and ΔE* increasing from 18.38 to 32.51. Short-term composting behavior was explored by embedding fragments from formulations with 40-60 wt.% total SCG + ALS (based on oven-dry fibers; equal SCG/ALS shares) into a mixed organic substrate adjusted to an initial C/N ≈ 30 and monitored for 30 days in pots and trays. The process remained predominantly mesophilic (≈14-22 °C); nevertheless, visible microbial colonization and progressive surface degradation were observed, indicating susceptibility to biological activity under moist, nutrient-rich conditions. Overall, the results show that SCG-ALS content strongly governs the visual identity of the biocomposites and suggest composting-oriented routes as a potential end-of-life direction at an exploratory level, while highlighting the need for standardized compostability assessment and longer-term monitoring to substantiate circularity claims.
Authors
- Petar Antov (ORCID: https://orcid.org/0000-0002-3837-5380)
- Georgi Ivanov
- Viktor Savov (ORCID: https://orcid.org/0000-0001-5111-8760)
- Ekaterina Ivanova‐Todorova (ORCID: https://orcid.org/0000-0002-1833-838X)
- Viktoria Dudeva (ORCID: https://orcid.org/0009-0003-0387-8716)
- Aleksandrina Kostadinova-Slaveva
- Jansu Yusein
- Boyka Malcheva
Institutions
- University of Forestry (BG)
- Sofia University "St. Kliment Ohridski" (BG)
Publication Details
- Journal
- Materials
- Published
- 2026-03-11
- DOI
- https://doi.org/10.3390/ma19061077
- Primary Topic
- Lignin and Wood Chemistry
- Type
- article
- Field-Weighted Citation Impact
- 0.00