Aesthetic Profiling and Exploratory Composting Screening of Wood-Fiber Biocomposites Bonded with Spent Coffee Grounds and Ammonium Lignosulfonate

Spent coffee grounds (SCGs) and lignin-derived binders, such as ammonium lignosulfonate (ALS), are increasingly being explored as renewable resources to reduce reliance on conventional formaldehyde-based resins in wood-fiber biocomposites. Although prior work has shown that SCG-ALS adhesive systems can achieve promising mechanical performance, two practical aspects essential for industrial applications and circular design remain insufficiently explored: a predictable and reproducible visual appearance and credible end-of-life options. In this study, sustainable wood-fiber biocomposites bonded with SCG and ALS were assessed from an aesthetic performance and end-of-life perspective. Color was quantified in the CIE L*a*b* (CIELAB) space and expressed as total color difference (ΔE*) relative to a reference panel. Increasing total SCG + ALS content from 40 to 75 wt.% based on oven-dry fibers produced pronounced darkening, with lightness decreasing from L* = 47.1 to 34.3 and ΔE* increasing from 18.38 to 32.51. Short-term composting behavior was explored by embedding fragments from formulations with 40-60 wt.% total SCG + ALS (based on oven-dry fibers; equal SCG/ALS shares) into a mixed organic substrate adjusted to an initial C/N ≈ 30 and monitored for 30 days in pots and trays. The process remained predominantly mesophilic (≈14-22 °C); nevertheless, visible microbial colonization and progressive surface degradation were observed, indicating susceptibility to biological activity under moist, nutrient-rich conditions. Overall, the results show that SCG-ALS content strongly governs the visual identity of the biocomposites and suggest composting-oriented routes as a potential end-of-life direction at an exploratory level, while highlighting the need for standardized compostability assessment and longer-term monitoring to substantiate circularity claims.

Authors

Institutions

Publication Details

Journal
Materials
Published
2026-03-11
DOI
https://doi.org/10.3390/ma19061077
Primary Topic
Lignin and Wood Chemistry
Type
article
Field-Weighted Citation Impact
0.00
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Aesthetic Profiling and Exploratory Composting Screening of Wood-Fiber Biocomposites Bonded with Spent Coffee Grounds and Ammonium Lignosulfonate

Petar Antov, Georgi Ivanov, Viktor Savov, Ekaterina Ivanova‐Todorova et al.
Materials
Lignin and Wood Chemistry
article

Aesthetic Profiling and Exploratory Composting Screening of Wood-Fiber Biocomposites Bonded with Spent Coffee Grounds and Ammonium Lignosulfonate

Petar Antov, Georgi Ivanov, Viktor Savov, Ekaterina Ivanova‐Todorova, Viktoria Dudeva, Aleksandrina Kostadinova-Slaveva, Jansu Yusein, Boyka Malcheva
article en

Abstract

Spent coffee grounds (SCGs) and lignin-derived binders, such as ammonium lignosulfonate (ALS), are increasingly being explored as renewable resources to reduce reliance on conventional formaldehyde-based resins in wood-fiber biocomposites. Although prior work has shown that SCG-ALS adhesive systems can achieve promising mechanical performance, two practical aspects essential for industrial applications and circular design remain insufficiently explored: a predictable and reproducible visual appearance and credible end-of-life options. In this study, sustainable wood-fiber biocomposites bonded with SCG and ALS were assessed from an aesthetic performance and end-of-life perspective. Color was quantified in the CIE L*a*b* (CIELAB) space and expressed as total color difference (ΔE*) relative to a reference panel. Increasing total SCG + ALS content from 40 to 75 wt.% based on oven-dry fibers produced pronounced darkening, with lightness decreasing from L* = 47.1 to 34.3 and ΔE* increasing from 18.38 to 32.51. Short-term composting behavior was explored by embedding fragments from formulations with 40-60 wt.% total SCG + ALS (based on oven-dry fibers; equal SCG/ALS shares) into a mixed organic substrate adjusted to an initial C/N ≈ 30 and monitored for 30 days in pots and trays. The process remained predominantly mesophilic (≈14-22 °C); nevertheless, visible microbial colonization and progressive surface degradation were observed, indicating susceptibility to biological activity under moist, nutrient-rich conditions. Overall, the results show that SCG-ALS content strongly governs the visual identity of the biocomposites and suggest composting-oriented routes as a potential end-of-life direction at an exploratory level, while highlighting the need for standardized compostability assessment and longer-term monitoring to substantiate circularity claims.

MaterialsVol. 19(6)
University of Forestry (BG), Sofia University "St. Kliment Ohridski" (BG)
Responsible consumption and production
Openalex Percentile: Top 25%
Lignin and Wood Chemistry
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.