Field-Programmable Topological Torons in Chiral Nematic Liquid Crystals

Torons are three-dimensional double-twist solitons in chiral nematic liquid crystals (LCs), bounded by closed defect loops, that behave as particle-like entities while retaining a fully reconfigurable optical response. Here, it is shown that individual torons can be created, translated, and parked on demand in planar antiparallel rubbed cells using a waveform-engineering approach. Torons are found to nucleate across a wide pitch window, set by the ratio of the cell gap to the chiral nematic pitch. Adjusting the voltage waveform parameters, namely, the modulation frequency, the duty-cycle asymmetry, and the addition of small DC offsets superimposed on a kilohertz carrier, results in programmable translation along eight in-plane directions within the LC cell. Transport is governed by two independently tunable channels: reorientation-driven backflow, which is dominant under time-balanced waveforms, and rectified polarity-sensitive coupling, activated by duty-cycle asymmetry. The drift direction can be reversed by changing the modulation conditions, even at zero offset, and a complementary reversal is observed when temperature is varied for fixed drive voltage conditions. Quantitative Landau-de Gennes Q-tensor simulations reproduce the equilibrium toron structure, its formation under the unmodulated carrier, and the relaxation pathway following field removal, while the transport mechanisms are identified from experimental signatures. A dedicated graphical interface enables real-time switching between waveform presets, and three proof-of-concept functions are demonstrated that exploit the resulting multiparameter control space: a software-defined racetrack memory analogue with optical readout, deterministic path writing for reconfigurable patterning, and toron-mediated pick-and-place transport of microparticles.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2026-09-18
DOI
https://doi.org/10.1021/acsami.6c10672
Primary Topic
Liquid Crystal Research Advancements
Type
article
Field-Weighted Citation Impact
0.00

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article

Field-Programmable Topological Torons in Chiral Nematic Liquid Crystals

Urban Mur, Waqas Kamal, Stephen Morris, Steve J. Elston et al.
ACS Applied Materials & Interfaces
Liquid Crystal Research Advancements
article

Field-Programmable Topological Torons in Chiral Nematic Liquid Crystals

Urban Mur, Waqas Kamal, Stephen Morris, Steve J. Elston, Jonghyeon Ka, Ji Qin, Adithya Pradeep, Tianxin Wang, Junseok Ma
article en

Abstract

Torons are three-dimensional double-twist solitons in chiral nematic liquid crystals (LCs), bounded by closed defect loops, that behave as particle-like entities while retaining a fully reconfigurable optical response. Here, it is shown that individual torons can be created, translated, and parked on demand in planar antiparallel rubbed cells using a waveform-engineering approach. Torons are found to nucleate across a wide pitch window, set by the ratio of the cell gap to the chiral nematic pitch. Adjusting the voltage waveform parameters, namely, the modulation frequency, the duty-cycle asymmetry, and the addition of small DC offsets superimposed on a kilohertz carrier, results in programmable translation along eight in-plane directions within the LC cell. Transport is governed by two independently tunable channels: reorientation-driven backflow, which is dominant under time-balanced waveforms, and rectified polarity-sensitive coupling, activated by duty-cycle asymmetry. The drift direction can be reversed by changing the modulation conditions, even at zero offset, and a complementary reversal is observed when temperature is varied for fixed drive voltage conditions. Quantitative Landau-de Gennes Q-tensor simulations reproduce the equilibrium toron structure, its formation under the unmodulated carrier, and the relaxation pathway following field removal, while the transport mechanisms are identified from experimental signatures. A dedicated graphical interface enables real-time switching between waveform presets, and three proof-of-concept functions are demonstrated that exploit the resulting multiparameter control space: a software-defined racetrack memory analogue with optical readout, deterministic path writing for reconfigurable patterning, and toron-mediated pick-and-place transport of microparticles.

ACS Applied Materials & Interfaces
University of Ljubljana (SI), Korea Advanced Institute of Science and Technology (KR), Korea Post (KR), University of Oxford (GB), Park University (US), Science Oxford (GB)
Engineering and Physical Sciences Research Council
Openalex Percentile: Top 89%
Liquid Crystal Research Advancements
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