Field-Programmable Topological Torons in Chiral Nematic Liquid Crystals
Torons are three-dimensional double-twist solitons in chiral nematic liquid crystals (LCs), bounded by closed defect loops, that behave as particle-like entities while retaining a fully reconfigurable optical response. Here, it is shown that individual torons can be created, translated, and parked on demand in planar antiparallel rubbed cells using a waveform-engineering approach. Torons are found to nucleate across a wide pitch window, set by the ratio of the cell gap to the chiral nematic pitch. Adjusting the voltage waveform parameters, namely, the modulation frequency, the duty-cycle asymmetry, and the addition of small DC offsets superimposed on a kilohertz carrier, results in programmable translation along eight in-plane directions within the LC cell. Transport is governed by two independently tunable channels: reorientation-driven backflow, which is dominant under time-balanced waveforms, and rectified polarity-sensitive coupling, activated by duty-cycle asymmetry. The drift direction can be reversed by changing the modulation conditions, even at zero offset, and a complementary reversal is observed when temperature is varied for fixed drive voltage conditions. Quantitative Landau-de Gennes Q-tensor simulations reproduce the equilibrium toron structure, its formation under the unmodulated carrier, and the relaxation pathway following field removal, while the transport mechanisms are identified from experimental signatures. A dedicated graphical interface enables real-time switching between waveform presets, and three proof-of-concept functions are demonstrated that exploit the resulting multiparameter control space: a software-defined racetrack memory analogue with optical readout, deterministic path writing for reconfigurable patterning, and toron-mediated pick-and-place transport of microparticles.
Authors
- Urban Mur (ORCID: https://orcid.org/0000-0003-3846-3839)
- Waqas Kamal (ORCID: https://orcid.org/0000-0001-6022-547X)
- Stephen Morris (ORCID: https://orcid.org/0000-0001-8294-9225)
- Steve J. Elston (ORCID: https://orcid.org/0000-0003-2719-539X)
- Jonghyeon Ka (ORCID: https://orcid.org/0000-0002-9203-224X)
- Ji Qin
- Adithya Pradeep
- Tianxin Wang
- Junseok Ma
Institutions
- University of Ljubljana (SI)
- Korea Advanced Institute of Science and Technology (KR)
- Korea Post (KR)
- University of Oxford (GB)
- Park University (US)
- Science Oxford (GB)
Publication Details
- Journal
- ACS Applied Materials & Interfaces
- Published
- 2026-09-18
- DOI
- https://doi.org/10.1021/acsami.6c10672
- Primary Topic
- Liquid Crystal Research Advancements
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Engineering and Physical Sciences Research Council