Laser-dressed ionic states in high-harmonic generation in helium

We report the experimental observation of an ionic resonance at 40.8 eV and two adjacent satellite sidebands in high-harmonic generation in neutral helium gas. The amplitude and asymmetry of the central line vary with different driving pulse intensities, which arises from the interference between the laser-dressed resonant emission from the 2 p state of He + ions and the nonresonant harmonic generation. The two satellite sidebands are identified as the virtual Floquet-like light-induced states located at ± ℏ ω d from the 2 s state of He + ions ( ω d denotes the driving laser frequency), whose multipeak profiles are imprinted by the structured spectrum of the driving laser pulse. These results demonstrate the roles of both bright and dark states of ionic species in shaping high-harmonic spectra in the vicinity of resonances.

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Publication Details

Journal
Optics Letters
Published
2026-03-05
DOI
https://doi.org/10.1364/ol.590912
Primary Topic
Laser-Matter Interactions and Applications
Type
article
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article

Laser-dressed ionic states in high-harmonic generation in helium

Lina Hedewig, Noah L. Wach, Gergana D. Borisova, Harijyoti Mandal et al.
Optics Letters
Laser-Matter Interactions and Applications
article

Laser-dressed ionic states in high-harmonic generation in helium

Lina Hedewig, Noah L. Wach, Gergana D. Borisova, Harijyoti Mandal, Yu He, Eleni Tzima, Thomas Pfeifer, Christian Ott
article en

Abstract

We report the experimental observation of an ionic resonance at 40.8 eV and two adjacent satellite sidebands in high-harmonic generation in neutral helium gas. The amplitude and asymmetry of the central line vary with different driving pulse intensities, which arises from the interference between the laser-dressed resonant emission from the 2 p state of He + ions and the nonresonant harmonic generation. The two satellite sidebands are identified as the virtual Floquet-like light-induced states located at ± ℏ ω d from the 2 s state of He + ions ( ω d denotes the driving laser frequency), whose multipeak profiles are imprinted by the structured spectrum of the driving laser pulse. These results demonstrate the roles of both bright and dark states of ionic species in shaping high-harmonic spectra in the vicinity of resonances.

Optics LettersVol. 51(7)
Max Planck Institute for Nuclear Physics (DE)
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Laser-Matter Interactions and Applications
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