In-Silicon Mietronics for Flatband-Enhanced Upconversion and Interfacial Loss Recovery

Silicon (Si) photodetectors exhibit limited infrared responsivity, restricting applications in communication, chemical sensing, and biomedical imaging. Although lanthanide-doped upconversion nanoparticles (UCNPs) can extend the spectral response of silicon, weak IR absorption and interfacial nonradiative losses have hindered etch-free monolithic integration. Here, we report an inverted-index UCNP-Si metasurface in which low-index NaYF<sub>4</sub>:Yb/Er nanocylinders are conformally coated with a high-index amorphous silicon layer. A collective-Mie flatband resonance at 976 nm enables near-unity absorption, simultaneously concentrating pump photons within the UCNP domains over a wide numerical aperture (NA ≈ 0.5) and activating near-field-mediated passivation of interfacial loss channels. The combined effects of resonant field enhancement and light-activated loss recovery yield a record 6800-fold increase in long-lived steady-state upconversion. This fully etch-free platform is compatible with complementary metal oxide semiconductor processing and provides a scalable route toward upconversion-enabled silicon photodetectors and compact light sources.

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Publication Details

Journal
Nano Letters
Published
2026-03-02
DOI
https://doi.org/10.1021/acs.nanolett.6c00215
Primary Topic
Luminescence Properties of Advanced Materials
Type
article
Field-Weighted Citation Impact
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article

In-Silicon Mietronics for Flatband-Enhanced Upconversion and Interfacial Loss Recovery

X Liu, Gianluigi Zito, Yuyang Gu, Yuxiang Zhang et al.
Nano Letters
Luminescence Properties of Advanced Materials
article

In-Silicon Mietronics for Flatband-Enhanced Upconversion and Interfacial Loss Recovery

X Liu, Gianluigi Zito, Yuyang Gu, Yuxiang Zhang, Febiana Tjiptoharsono, Sourav Adhikary, Mengfei Wu
article en

Abstract

Silicon (Si) photodetectors exhibit limited infrared responsivity, restricting applications in communication, chemical sensing, and biomedical imaging. Although lanthanide-doped upconversion nanoparticles (UCNPs) can extend the spectral response of silicon, weak IR absorption and interfacial nonradiative losses have hindered etch-free monolithic integration. Here, we report an inverted-index UCNP-Si metasurface in which low-index NaYF<sub>4</sub>:Yb/Er nanocylinders are conformally coated with a high-index amorphous silicon layer. A collective-Mie flatband resonance at 976 nm enables near-unity absorption, simultaneously concentrating pump photons within the UCNP domains over a wide numerical aperture (NA ≈ 0.5) and activating near-field-mediated passivation of interfacial loss channels. The combined effects of resonant field enhancement and light-activated loss recovery yield a record 6800-fold increase in long-lived steady-state upconversion. This fully etch-free platform is compatible with complementary metal oxide semiconductor processing and provides a scalable route toward upconversion-enabled silicon photodetectors and compact light sources.

Nano LettersVol. 26(9)
Agency for Science, Technology and Research (SG), National University of Singapore (SG), Institute of Applied Science and Intelligent Systems (IT), Institute of Materials Research and Engineering (SG)
Industry, innovation and infrastructure
Openalex Percentile: Top 40%
Luminescence Properties of Advanced Materials
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In-Silicon Mietronics for Flatband-Enhanced Upconversion and Interfacial Loss Recovery — X Liu, Gianluigi Zito, et al. · Nano Letters (2026) | TGRS Research Map | TGRS