In-Silicon Mietronics for Flatband-Enhanced Upconversion and Interfacial Loss Recovery
Silicon (Si) photodetectors exhibit limited infrared responsivity, restricting applications in communication, chemical sensing, and biomedical imaging. Although lanthanide-doped upconversion nanoparticles (UCNPs) can extend the spectral response of silicon, weak IR absorption and interfacial nonradiative losses have hindered etch-free monolithic integration. Here, we report an inverted-index UCNP-Si metasurface in which low-index NaYF<sub>4</sub>:Yb/Er nanocylinders are conformally coated with a high-index amorphous silicon layer. A collective-Mie flatband resonance at 976 nm enables near-unity absorption, simultaneously concentrating pump photons within the UCNP domains over a wide numerical aperture (NA ≈ 0.5) and activating near-field-mediated passivation of interfacial loss channels. The combined effects of resonant field enhancement and light-activated loss recovery yield a record 6800-fold increase in long-lived steady-state upconversion. This fully etch-free platform is compatible with complementary metal oxide semiconductor processing and provides a scalable route toward upconversion-enabled silicon photodetectors and compact light sources.
Authors
- X Liu
- Gianluigi Zito (ORCID: https://orcid.org/0000-0003-2376-0080)
- Yuyang Gu (ORCID: https://orcid.org/0000-0002-0826-1868)
- Yuxiang Zhang (ORCID: https://orcid.org/0000-0001-9047-9585)
- Febiana Tjiptoharsono (ORCID: https://orcid.org/0009-0002-7176-6479)
- Sourav Adhikary
- Mengfei Wu
Institutions
- Agency for Science, Technology and Research (SG)
- National University of Singapore (SG)
- Institute of Applied Science and Intelligent Systems (IT)
- Institute of Materials Research and Engineering (SG)
Publication Details
- Journal
- Nano Letters
- Published
- 2026-03-02
- DOI
- https://doi.org/10.1021/acs.nanolett.6c00215
- Primary Topic
- Luminescence Properties of Advanced Materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00