On-Chip Plasmonic Slit-Cavity Platform for Room-Temperature Strong Coupling with Deterministically Positioned Colloidal Quantum Dots

Strong coupling between quantum emitters and optical cavities underpins many quantum photonic technologies, yet achieving this regime at room temperature in compact, deterministic on-chip platforms remains challenging due to the difficulty of fabricating cavities with ultrasmall mode volumes and precisely positioning quantum emitters. Here, we demonstrate a robust quantum plasmonic device in which colloidal quantum dots are strongly coupled to plasmonic slit cavities. Our dielectrophoresis-based positioning technique with real-time photoluminescence feedback enables parallel device fabrication and straightforward integration with additional optical elements, such as waveguides. Our measurements reveal clear photoluminescence-resolved Rabi splitting at room temperature in precharacterized cavities, with device-to-device variations scaling with the average number of coupled quantum dots. While electrical tuning via the quantum-confined Stark effect is enabled by integrated electrodes, its impact is largely overshadowed by room-temperature spectral diffusion. These results establish a scalable and electrically addressable plasmonic platform for room-temperature quantum technologies.

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Publication Details

Journal
Nano Letters
Published
2026-02-27
DOI
https://doi.org/10.1021/acs.nanolett.5c05910
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
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article

On-Chip Plasmonic Slit-Cavity Platform for Room-Temperature Strong Coupling with Deterministically Positioned Colloidal Quantum Dots

P. Pertsch, A. Podhorodecki, Benedikt Schurr, Bert Hecht et al.
Nano Letters
Plasmonic and Surface Plasmon Research
article

On-Chip Plasmonic Slit-Cavity Platform for Room-Temperature Strong Coupling with Deterministically Positioned Colloidal Quantum Dots

P. Pertsch, A. Podhorodecki, Benedikt Schurr, Bert Hecht, Monika Emmerling, Max Knopf, Saeid Asgarnezhad-Zorgabad, Lars Meschede, Jin Qin, Ortwin Hess, Daniel D. A. Clarke, Daniel Friedrich
article en

Abstract

Strong coupling between quantum emitters and optical cavities underpins many quantum photonic technologies, yet achieving this regime at room temperature in compact, deterministic on-chip platforms remains challenging due to the difficulty of fabricating cavities with ultrasmall mode volumes and precisely positioning quantum emitters. Here, we demonstrate a robust quantum plasmonic device in which colloidal quantum dots are strongly coupled to plasmonic slit cavities. Our dielectrophoresis-based positioning technique with real-time photoluminescence feedback enables parallel device fabrication and straightforward integration with additional optical elements, such as waveguides. Our measurements reveal clear photoluminescence-resolved Rabi splitting at room temperature in precharacterized cavities, with device-to-device variations scaling with the average number of coupled quantum dots. While electrical tuning via the quantum-confined Stark effect is enabled by integrated electrodes, its impact is largely overshadowed by room-temperature spectral diffusion. These results establish a scalable and electrically addressable plasmonic platform for room-temperature quantum technologies.

Nano LettersVol. 26(11)
Wrocław University of Science and Technology (PL), Trinity College Dublin (IE), University of Würzburg (DE), AGH University of Krakow (PL)
Affordable and clean energy
Openalex Percentile: Top 43%
Plasmonic and Surface Plasmon Research
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