Charge density fluctuations uncover the relevance of electron-phonon coupling in cuprate superconductors

Abstract Electron–phonon coupling (EPC) is a key interaction governing lattice dynamics, charge transport, and collective electronic phases in quantum materials. In several families of unconventional superconductors, including transition-metal dichalcogenides and kagome metals, growing evidence points to a cooperative role of EPC and dynamic charge density fluctuations (CDF) in stabilizing superconductivity. Yet, how the strength of EPC evolves across phase diagrams and relates to superconducting properties in strongly correlated systems remains an open question. Here we investigate the interplay between phonons and the CDF recently identified in cuprate superconductors. Using resonant inelastic x-ray scattering, we track the dispersion and intensity of bond-stretching phonons in YBa 2 Cu 3 O 7− δ over wide ranges of doping, temperature, and momentum. We observe that both the phonon softening at the CDF wave vector and the effective charge–lattice response probed by the RIXS phonon intensity are maximized near p = 0.19, where superconducting properties are optimal and CDF intensity is strongest. These results identify dynamic charge density fluctuations, rather than static charge density waves, as the dominant source of phonon renormalization in cuprates, and establish a direct correlation between the EPC-related phonon renormalization and the superconducting dome. More broadly, our measurements emphasize EPC as a doping dependent property of correlated materials, shaped by the electronic environment in which lattice vibrations are embedded.

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Journal
Communications Materials
Published
2026-11-03
DOI
https://doi.org/10.1038/s43246-026-01413-5
Primary Topic
Physics of Superconductivity and Magnetism
Type
article
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article

Charge density fluctuations uncover the relevance of electron-phonon coupling in cuprate superconductors

M. Moretti Sala, Giacomo Claudio Ghiringhelli, Riccardo Arpaia, Nicholas B. Brookes et al.
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Communications Materials
Physics of Superconductivity and Magnetism
article

Charge density fluctuations uncover the relevance of electron-phonon coupling in cuprate superconductors

M. Moretti Sala, Giacomo Claudio Ghiringhelli, Riccardo Arpaia, Nicholas B. Brookes, Floriana Lombardi, S. Caprara, Giacomo Merzoni, F. Rosa, Martina Fedele
article en

Abstract

Abstract Electron–phonon coupling (EPC) is a key interaction governing lattice dynamics, charge transport, and collective electronic phases in quantum materials. In several families of unconventional superconductors, including transition-metal dichalcogenides and kagome metals, growing evidence points to a cooperative role of EPC and dynamic charge density fluctuations (CDF) in stabilizing superconductivity. Yet, how the strength of EPC evolves across phase diagrams and relates to superconducting properties in strongly correlated systems remains an open question. Here we investigate the interplay between phonons and the CDF recently identified in cuprate superconductors. Using resonant inelastic x-ray scattering, we track the dispersion and intensity of bond-stretching phonons in YBa 2 Cu 3 O 7− δ over wide ranges of doping, temperature, and momentum. We observe that both the phonon softening at the CDF wave vector and the effective charge–lattice response probed by the RIXS phonon intensity are maximized near p = 0.19, where superconducting properties are optimal and CDF intensity is strongest. These results identify dynamic charge density fluctuations, rather than static charge density waves, as the dominant source of phonon renormalization in cuprates, and establish a direct correlation between the EPC-related phonon renormalization and the superconducting dome. More broadly, our measurements emphasize EPC as a doping dependent property of correlated materials, shaped by the electronic environment in which lattice vibrations are embedded.

Communications Materials
Ca' Foscari University of Venice (IT), European Synchrotron Radiation Facility (FR), Chalmers University of Technology (SE), Sapienza University of Rome (IT), European X-Ray Free-Electron Laser (DE), Politecnico di Milano (IT)
Openalex Percentile: Top 88%
Physics of Superconductivity and Magnetism
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