Aging of amorphous materials under cyclic strain

Amorphous materials driven away from equilibrium display a diverse repertoire of complex, history-dependent behaviors. One striking feature is a failure to return to equilibrium after an abrupt change in otherwise static external conditions. Instead, amorphous materials often exhibit physical aging: an ever-slowing, nonexponential relaxation that can span a huge range of timescales. Here, we examine the aging behavior of three different amorphous materials subjected to slow periodic driving. The results reveal a generic aging phenomenon characterized by a logarithmic decay of dissipation per cycle. This observation is evaluated against several mesoscopic models of amorphous matter that successfully capture aging under static conditions: i) a collection of noninteracting relaxation processes ii) a noisy hysteron model with random pairwise interactions, and iii) a structural model consisting of a random network of bistable elastic bonds. We find that only the latter model reproduces all experimental findings and relates its success to its persistent, slow exploration of a complex energy landscape with clear signatures of replica symmetry breaking. Thus, cyclic driving emerges as a simple yet powerful protocol to characterize amorphous materials, probe their complex energy landscapes, and distinguish between different models.

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Publication Details

Journal
Proceedings of the National Academy of Sciences
Published
2026-02-18
DOI
https://doi.org/10.1073/pnas.2515075123
Citations
1
Primary Topic
Material Dynamics and Properties
Type
article
Field-Weighted Citation Impact
16.08
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article

Aging of amorphous materials under cyclic strain

Martin van Hecke, Paul Baconnier, Dor Shohat, Yoav Lahini et al.
1 citations
Proceedings of the National Academy of Sciences
Material Dynamics and Properties
16.08
article

Aging of amorphous materials under cyclic strain

Martin van Hecke, Paul Baconnier, Dor Shohat, Yoav Lahini, Itamar Procaccia
article en
1 citations

Abstract

Amorphous materials driven away from equilibrium display a diverse repertoire of complex, history-dependent behaviors. One striking feature is a failure to return to equilibrium after an abrupt change in otherwise static external conditions. Instead, amorphous materials often exhibit physical aging: an ever-slowing, nonexponential relaxation that can span a huge range of timescales. Here, we examine the aging behavior of three different amorphous materials subjected to slow periodic driving. The results reveal a generic aging phenomenon characterized by a logarithmic decay of dissipation per cycle. This observation is evaluated against several mesoscopic models of amorphous matter that successfully capture aging under static conditions: i) a collection of noninteracting relaxation processes ii) a noisy hysteron model with random pairwise interactions, and iii) a structural model consisting of a random network of bistable elastic bonds. We find that only the latter model reproduces all experimental findings and relates its success to its persistent, slow exploration of a complex energy landscape with clear signatures of replica symmetry breaking. Thus, cyclic driving emerges as a simple yet powerful protocol to characterize amorphous materials, probe their complex energy landscapes, and distinguish between different models.

Proceedings of the National Academy of SciencesVol. 123(8)
Leiden University (NL), North University of China (CN), Tel Aviv University (IL), Huygens Institute for History and Culture of the Netherlands (NL), Institute for Atomic and Molecular Physics (NL), Faculty (United Kingdom) (GB), Civilisations Matter (DE), Complexity Science Hub (AT), Living Systems (United States) (US), Weizmann Institute of Science (IL)
Affordable and clean energy
Openalex Percentile: Top 1%
Material Dynamics and Properties
16.08
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Aging of amorphous materials under cyclic strain — Martin van Hecke, Paul Baconnier, et al. · Proceedings of the National Academy of Sciences (2026) | TGRS Research Map | TGRS