Aging of amorphous materials under cyclic strain
Amorphous materials driven away from equilibrium display a diverse repertoire of complex, history-dependent behaviors. One striking feature is a failure to return to equilibrium after an abrupt change in otherwise static external conditions. Instead, amorphous materials often exhibit physical aging: an ever-slowing, nonexponential relaxation that can span a huge range of timescales. Here, we examine the aging behavior of three different amorphous materials subjected to slow periodic driving. The results reveal a generic aging phenomenon characterized by a logarithmic decay of dissipation per cycle. This observation is evaluated against several mesoscopic models of amorphous matter that successfully capture aging under static conditions: i) a collection of noninteracting relaxation processes ii) a noisy hysteron model with random pairwise interactions, and iii) a structural model consisting of a random network of bistable elastic bonds. We find that only the latter model reproduces all experimental findings and relates its success to its persistent, slow exploration of a complex energy landscape with clear signatures of replica symmetry breaking. Thus, cyclic driving emerges as a simple yet powerful protocol to characterize amorphous materials, probe their complex energy landscapes, and distinguish between different models.
Authors
- Martin van Hecke (ORCID: https://orcid.org/0000-0002-9550-6607)
- Paul Baconnier (ORCID: https://orcid.org/0000-0003-3526-7605)
- Dor Shohat (ORCID: https://orcid.org/0000-0003-4573-238X)
- Yoav Lahini
- Itamar Procaccia
Institutions
- Leiden University (NL)
- North University of China (CN)
- Tel Aviv University (IL)
- Huygens Institute for History and Culture of the Netherlands (NL)
- Institute for Atomic and Molecular Physics (NL)
- Faculty (United Kingdom) (GB)
- Civilisations Matter (DE)
- Complexity Science Hub (AT)
- Living Systems (United States) (US)
- Weizmann Institute of Science (IL)
Publication Details
- Journal
- Proceedings of the National Academy of Sciences
- Published
- 2026-02-18
- DOI
- https://doi.org/10.1073/pnas.2515075123
- Citations
- 1
- Primary Topic
- Material Dynamics and Properties
- Type
- article
- Field-Weighted Citation Impact
- 16.08