Anthropogenic Oxygenated Organic Molecules Dominate New Particle Growth in Moderate-Pollution Urban China

New particle formation (NPF) represents a major aerosol source with profound implications for air quality and global climate. While studies in heavily polluted megacities (e.g., Beijing) have typically revealed high nucleation rates coupled with slow particle growth, the mechanisms governing NPF under moderate pollution regimes remain poorly understood. Here, we report a distinct NPF pattern in the coastal city of Xiamen, characterized by relatively low nucleation rates but exceptionally rapid particle growth. Field observations and model simulations show that anthropogenic oxygenated organic molecules (OOMs), rather than sulfuric acid, dominate particle growth from the sub-3 nm size range. Despite a modest nucleation rate (<i>J</i><sub>1.7</sub> = 1.2 cm<sup>3</sup> s<sup>-1</sup>), the observed high growth rate (GR<sub>7-15</sub> = 7.2 nm h<sup>-1</sup>) is largely attributable to condensable organic vapors from anthropogenic sources. This efficient, anthropogenically driven growth pathway suggests that NPF could play a more substantial role in aerosol formation in many moderately polluted urban environments than currently recognized. We therefore urge the integration of such anthropogenic organic-driven growth mechanisms into atmospheric models to improve climate predictions.

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Publication Details

Journal
Environmental Science & Technology
Published
2026-02-18
DOI
https://doi.org/10.1021/acs.est.5c11555
Primary Topic
Atmospheric chemistry and aerosols
Type
article
Field-Weighted Citation Impact
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article

Anthropogenic Oxygenated Organic Molecules Dominate New Particle Growth in Moderate-Pollution Urban China

Ziyi Lin, G. Y. Chen, Runlong Cai, James Brean et al.
Environmental Science & Technology
Atmospheric chemistry and aerosols
article

Anthropogenic Oxygenated Organic Molecules Dominate New Particle Growth in Moderate-Pollution Urban China

Ziyi Lin, G. Y. Chen, Runlong Cai, James Brean, Lingjun Li, Yuping Chen, Jinsheng Chen, Yunxiang Zhang, Mengren Li, Wei Huang, Chen Yang, Wei Du, Lingling Xu, Wei Xu, Xiaolong Fan
article en

Abstract

New particle formation (NPF) represents a major aerosol source with profound implications for air quality and global climate. While studies in heavily polluted megacities (e.g., Beijing) have typically revealed high nucleation rates coupled with slow particle growth, the mechanisms governing NPF under moderate pollution regimes remain poorly understood. Here, we report a distinct NPF pattern in the coastal city of Xiamen, characterized by relatively low nucleation rates but exceptionally rapid particle growth. Field observations and model simulations show that anthropogenic oxygenated organic molecules (OOMs), rather than sulfuric acid, dominate particle growth from the sub-3 nm size range. Despite a modest nucleation rate (<i>J</i><sub>1.7</sub> = 1.2 cm<sup>3</sup> s<sup>-1</sup>), the observed high growth rate (GR<sub>7-15</sub> = 7.2 nm h<sup>-1</sup>) is largely attributable to condensable organic vapors from anthropogenic sources. This efficient, anthropogenically driven growth pathway suggests that NPF could play a more substantial role in aerosol formation in many moderately polluted urban environments than currently recognized. We therefore urge the integration of such anthropogenic organic-driven growth mechanisms into atmospheric models to improve climate predictions.

Environmental Science & TechnologyVol. 60(8)
University of Helsinki (FI), Chinese Academy of Sciences (CN), Fudan University (CN), Paul Scherrer Institute (CH), State Key Laboratory of Pollution Control and Resource Reuse (CN), Institute of Urban Environment (CN), Department of Chemistry and Earth Sciences (BY), Environmental Earth Sciences (AU), University of Chinese Academy of Sciences (CN), University of Birmingham (GB)
Climate action
Openalex Percentile: Top 64%
Atmospheric chemistry and aerosols
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