Spin–Orbit-Torque-Driven Terahertz Oscillations in Pt/KFe <sub>3</sub> (OH) <sub>6</sub> (SO <sub>4</sub> ) <sub>2</sub> /W Trilayer Structure

We propose a nanoscale terahertz (THz) signal generator based on a Pt/KFe<sub>3</sub>(OH)<sub>6</sub>(SO<sub>4</sub>)<sub>2</sub>/W trilayer structure that produces stable THz output under direct-current driving. Spin currents injected from the Pt layer generate spin-orbit torque (SOT), exciting the magnetic moments of the noncollinear antiferromagnet (AFM) KFe<sub>3</sub>(OH)<sub>6</sub>(SO<sub>4</sub>)<sub>2</sub> and inducing steady magnetization oscillations. These oscillations generate THz alternating-current (AC) signals, which are electrically detected via the inverse spin Hall effect (ISHE) in the W layer. The asymmetric heavy-metal/AFM/heavy-metal configuration, featuring opposite spin Hall angles, enables efficient spin-current injection and signal readout. Micromagnetic simulations and theoretical analysis reveal that the THz signal originates from the asymmetric distribution of Dzyaloshinskii-Moriya interaction (DMI) energy. A quantitative relationship between excitation current and signal output is established, and tunable frequency control with reduced threshold current is achieved by optimizing material and structural parameters.

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Publication Details

Journal
The Journal of Physical Chemistry Letters
Published
2026-02-17
DOI
https://doi.org/10.1021/acs.jpclett.5c04101
Primary Topic
Magnetic properties of thin films
Type
article
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article

Spin–Orbit-Torque-Driven Terahertz Oscillations in Pt/KFe 3 (OH) 6 (SO 4 ) 2 /W Trilayer Structure

Boshi Mu, Yan Liu, Xiaofeng Cheng
The Journal of Physical Chemistry Letters
Magnetic properties of thin films
article

Spin–Orbit-Torque-Driven Terahertz Oscillations in Pt/KFe 3 (OH) 6 (SO 4 ) 2 /W Trilayer Structure

Boshi Mu, Yan Liu, Xiaofeng Cheng
article en

Abstract

We propose a nanoscale terahertz (THz) signal generator based on a Pt/KFe<sub>3</sub>(OH)<sub>6</sub>(SO<sub>4</sub>)<sub>2</sub>/W trilayer structure that produces stable THz output under direct-current driving. Spin currents injected from the Pt layer generate spin-orbit torque (SOT), exciting the magnetic moments of the noncollinear antiferromagnet (AFM) KFe<sub>3</sub>(OH)<sub>6</sub>(SO<sub>4</sub>)<sub>2</sub> and inducing steady magnetization oscillations. These oscillations generate THz alternating-current (AC) signals, which are electrically detected via the inverse spin Hall effect (ISHE) in the W layer. The asymmetric heavy-metal/AFM/heavy-metal configuration, featuring opposite spin Hall angles, enables efficient spin-current injection and signal readout. Micromagnetic simulations and theoretical analysis reveal that the THz signal originates from the asymmetric distribution of Dzyaloshinskii-Moriya interaction (DMI) energy. A quantitative relationship between excitation current and signal output is established, and tunable frequency control with reduced threshold current is achieved by optimizing material and structural parameters.

The Journal of Physical Chemistry LettersVol. 17(8)
College of Medical Sciences (NP), Universidad del Noreste (MX)
Affordable and clean energy
Openalex Percentile: Top 51%
Magnetic properties of thin films
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