Diameter-Controlled High-Order Vortex States and Magnon Hybridization in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>VSe</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:

Curved magnets offer a rich phase diagram and hold great promise for next-generation spintronic technologies. This Letter establishes the paramount significance of high-order vortex states (e.g., 3φ with winding number n≥2) in VSe_{2} nanotubes, which uniquely enable magnonic functionalities fundamentally inaccessible to conventional magnetic systems, and additionally, the superposition of high-order vortex and helical states is identified. These states arise from diameter-dependent competition between the nearest-neighbor ferromagnetic (J_{1}) and longer-range antiferromagnetic (J_{2}/J_{3}) couplings, as jointly validated through density-functional theory calculations and Heisenberg modeling of phase diagrams. Based on the Landau-Lifshitz-Gilbert equation, we show that vortex states exhibit orbital angular momentum (OAM) hybridization governed by selection rules: magnetic anisotropy energy (MAE) and an external magnetic field couple the l mode to l±2(n1) and l±n, respectively. For the 3φ state, MAE couples the l=0 mode with l=±4, producing eight-petal magnon density patterns and providing a natural mechanism for generating high-OAM magnons. These findings establish a predictive theoretical framework for controlling high-order vortex states in curved magnets and highlight VSe_{2} nanotubes as a promising platform for exploring complex magnetism and for the development of future magnonic and spintronic devices.

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Publication Details

Journal
Physical Review Letters
Published
2026-02-13
DOI
https://doi.org/10.1103/jr3h-1674
Primary Topic
2D Materials and Applications
Type
article
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Diameter-Controlled High-Order Vortex States and Magnon Hybridization in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>VSe</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:

Bo Zhong Gu, Jin Zhang, Anonymous, Xin-Wei Yi et al.
Physical Review Letters
2D Materials and Applications
article

Diameter-Controlled High-Order Vortex States and Magnon Hybridization in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>VSe</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:

Bo Zhong Gu, Jin Zhang, Anonymous, Xin-Wei Yi, Gang Su
article en

Abstract

Curved magnets offer a rich phase diagram and hold great promise for next-generation spintronic technologies. This Letter establishes the paramount significance of high-order vortex states (e.g., 3φ with winding number n≥2) in VSe_{2} nanotubes, which uniquely enable magnonic functionalities fundamentally inaccessible to conventional magnetic systems, and additionally, the superposition of high-order vortex and helical states is identified. These states arise from diameter-dependent competition between the nearest-neighbor ferromagnetic (J_{1}) and longer-range antiferromagnetic (J_{2}/J_{3}) couplings, as jointly validated through density-functional theory calculations and Heisenberg modeling of phase diagrams. Based on the Landau-Lifshitz-Gilbert equation, we show that vortex states exhibit orbital angular momentum (OAM) hybridization governed by selection rules: magnetic anisotropy energy (MAE) and an external magnetic field couple the l mode to l±2(n1) and l±n, respectively. For the 3φ state, MAE couples the l=0 mode with l=±4, producing eight-petal magnon density patterns and providing a natural mechanism for generating high-OAM magnons. These findings establish a predictive theoretical framework for controlling high-order vortex states in curved magnets and highlight VSe_{2} nanotubes as a promising platform for exploring complex magnetism and for the development of future magnonic and spintronic devices.

Physical Review LettersVol. 136(9)
Center for NanoScience (DE), Kavli Institute for Theoretical Sciences (CN), Institute of Theoretical Physics (CN), National Center for Nanoscience and Technology (CN), University of Chinese Academy of Sciences (CN)
Openalex Percentile: Top 57%
2D Materials and Applications
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