Magnetic excitations in the Kitaev material <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Na</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>IrO</mml:mi> <mml:mn>3</mml:mn> </mml:msub> </mml:mrow>

Inelastic neutron scattering experiments with a large set of comounted Na$_2$IrO$_3$ crystals reveal the low-energy magnon dispersion in this candidate material for Kitaev physics. The magnon gap amounts to 1.7(1) meV and can be interpreted similarly to the sister compound $α$-RuCl$_{3}$ to stem from the zone boundaries in the antiferromagnetic zigzag structure. The neutron experiments find no evidence for low-energy excitations with ferromagnetic character, which contrasts to the findings in $α$-RuCl$_{3}$. Our results are consistent with a recently proposed microscopic model that involves an antiferromagnetic Heisenberg nearest-neighbor exchange in Na$_2$IrO$_3$ in contrast to the ferromagnetic one considered for $α$-RuCl$_{3}$. Although the magnetic response shows the signatures of bond-directional anisotropy in both materials the different relative signs of Kitaev and Heisenberg interaction result in different deviations from the initial Kitaev model. Low-energy ferromagnetic fluctuations cannot be considered as a fingerprint of ferromagnetic Kitaev interaction.

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Journal
Physical review. B./Physical review. B
Published
2026-02-11
DOI
https://doi.org/10.1103/mvn9-nj5n
Primary Topic
Advanced Condensed Matter Physics
Type
article
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article

Magnetic excitations in the Kitaev material <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Na</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>IrO</mml:mi> <mml:mn>3</mml:mn> </mml:msub> </mml:mrow>

A. Ivanov, Hengdi Zhao, Andrea Piovano, M. Braden et al.
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
article

Magnetic excitations in the Kitaev material <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Na</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>IrO</mml:mi> <mml:mn>3</mml:mn> </mml:msub> </mml:mrow>

A. Ivanov, Hengdi Zhao, Andrea Piovano, M. Braden, Gang Cao, Anonymous, Paul Steffens
article en

Abstract

Inelastic neutron scattering experiments with a large set of comounted Na$_2$IrO$_3$ crystals reveal the low-energy magnon dispersion in this candidate material for Kitaev physics. The magnon gap amounts to 1.7(1) meV and can be interpreted similarly to the sister compound $α$-RuCl$_{3}$ to stem from the zone boundaries in the antiferromagnetic zigzag structure. The neutron experiments find no evidence for low-energy excitations with ferromagnetic character, which contrasts to the findings in $α$-RuCl$_{3}$. Our results are consistent with a recently proposed microscopic model that involves an antiferromagnetic Heisenberg nearest-neighbor exchange in Na$_2$IrO$_3$ in contrast to the ferromagnetic one considered for $α$-RuCl$_{3}$. Although the magnetic response shows the signatures of bond-directional anisotropy in both materials the different relative signs of Kitaev and Heisenberg interaction result in different deviations from the initial Kitaev model. Low-energy ferromagnetic fluctuations cannot be considered as a fingerprint of ferromagnetic Kitaev interaction.

Physical review. B./Physical review. BVol. 113(9)
University of Cologne (DE), University of Colorado System (US), Institut Laue-Langevin (FR)
Openalex Percentile: Top 57%
Advanced Condensed Matter Physics
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