Variation in Fine Particulate Matter Exposure Models: Implications for Health, Equity, and Uncertainty Evaluation

We seek to understand how uncertainty in spatiotemporal models of PM2.5 concentration influences exposure, equity, and health metrics in Canada. We evaluated the accuracy of seven longitudinal PM2.5 concentration data sets from 2002 to 2014 and conducted equity and health impact analysis using each. Specifically, we estimated population exposure improvements over time, exposure disparities for vulnerable subpopulations, and PM2.5-attributable mortality across several combinations of inputs. Nationally, reductions in population exposure to PM2.5 were consistently observed in all models between 2002 and 2014 in Canada, with larger reductions among subpopulations of visible minority status, suggesting that PM2.5 exposure and absolute exposure disparities improved over this period. Agreement between PM2.5 models is strongest for PM2.5-attributable mortality, whereas exposure time trends and contrasts between subpopulations differ more widely. Nationally, estimated PM2.5-attributable mortality ranged from 7,400 to 26,000 deaths in 2014 across combinations of seven PM2.5 models, four Canadian risk estimates, and counterfactuals of 0 and 2.5 μg/m3. PM2.5-attributable death estimates are sensitive to inputs of mortality risks, counterfactuals, and PM2.5 models. Improving estimates of Canadian PM2.5 exposure remains important for reducing uncertainty in health studies, particularly for accountability, equity, and epidemiological studies that rely on spatial or temporal contrasts.

Authors

Institutions

Publication Details

Journal
ACS ES&T Air
Published
2026-02-05
DOI
https://doi.org/10.1021/acsestair.5c00330
Primary Topic
Air Quality and Health Impacts
Type
article
Field-Weighted Citation Impact
0.00
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Variation in Fine Particulate Matter Exposure Models: Implications for Health, Equity, and Uncertainty Evaluation

Maxim Bulat, Elysia G. Fuller-Thomson, H Chen, Amanda J. Pappin et al.
ACS ES&T Air
Air Quality and Health Impacts
article

Variation in Fine Particulate Matter Exposure Models: Implications for Health, Equity, and Uncertainty Evaluation

Maxim Bulat, Elysia G. Fuller-Thomson, H Chen, Amanda J. Pappin, Nedka Pentcheva, Saeed Nadi, Xihong Wang, Anas Alhusban, A. Hakami, Richard T. Burnett, Y. Burak Oztaner
article en

Abstract

We seek to understand how uncertainty in spatiotemporal models of PM2.5 concentration influences exposure, equity, and health metrics in Canada. We evaluated the accuracy of seven longitudinal PM2.5 concentration data sets from 2002 to 2014 and conducted equity and health impact analysis using each. Specifically, we estimated population exposure improvements over time, exposure disparities for vulnerable subpopulations, and PM2.5-attributable mortality across several combinations of inputs. Nationally, reductions in population exposure to PM2.5 were consistently observed in all models between 2002 and 2014 in Canada, with larger reductions among subpopulations of visible minority status, suggesting that PM2.5 exposure and absolute exposure disparities improved over this period. Agreement between PM2.5 models is strongest for PM2.5-attributable mortality, whereas exposure time trends and contrasts between subpopulations differ more widely. Nationally, estimated PM2.5-attributable mortality ranged from 7,400 to 26,000 deaths in 2014 across combinations of seven PM2.5 models, four Canadian risk estimates, and counterfactuals of 0 and 2.5 μg/m3. PM2.5-attributable death estimates are sensitive to inputs of mortality risks, counterfactuals, and PM2.5 models. Improving estimates of Canadian PM2.5 exposure remains important for reducing uncertainty in health studies, particularly for accountability, equity, and epidemiological studies that rely on spatial or temporal contrasts.

ACS ES&T AirVol. 3(3)
Health Canada (CA), North Carolina Department of Environmental Quality (US), Environment and Climate Change Canada (CA), India Meteorological Department (IN), Carleton University (CA)
Good health and well-being
Openalex Percentile: Top 66%
Air Quality and Health Impacts
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.