Proton-Fluid Preintercalation Topochemistry for High-Rate Capacity and Ultralow-Temperature Proton Storage
Fundamental limitations in structural reversibility and electrochemical performance have rendered anode materials a critical bottleneck for proton batteries and capacitors. While the rational design of intrinsic properties for metal oxides offers a promising route for advanced proton storage, the simultaneous realization of high-power and low-temperature operability remains a grand challenge. We show that topochemical preintercalation of protons and confined lattice water in hydrated molybdenum bronze modifies host lattice rearrangement and enables ultrafast proton-coupled electron transfer. Ion-fluid cointercalation mediates electrochemical reaction pathways to an unconventional three-proton insertion mechanism, enabling a state-of-the-art specific capacity of 407 mAh g<sup>-1</sup>, ultrahigh-rate capability exceeding 1000 C (500 A g<sup>-1</sup>), and ultralow-temperature adaptability (194.2 mAh g<sup>-1</sup> at -80 °C). Comprehensive in situ crystal and interface evolution methods and theoretical calculations reveal a highly reversible and homogeneous protonation mechanism and enhanced interfacial transport, suppressing heterogeneous and unstable reaction kinetics of pristine MoO<sub>3</sub>. The hybrid proton capacitor with such a molybdenum bronze anode shows an unprecedented ultrahigh-power and ultralow-temperature performance, with excellent stability for over 2000 cycles at -80 °C. This work highlights physicochemical insights on preintercalation topochemistry in modulating charge carrier-host interactions and provides electrode design principles for high-rate and low-temperature nonmetallic ion storage.
Authors
- Tengyu Yao
- Kongjun Zhu
- Yuxuan Zhao
- Zhenhui Liu (ORCID: https://orcid.org/0000-0001-7001-6006)
- Laifa Shen
- Tiezhu Xu
- Zhenming Xu
- Duo Chen
Institutions
- Energy Storage Systems (United States) (US)
- Nanjing University of Aeronautics and Astronautics (CN)
Publication Details
- Journal
- Journal of the American Chemical Society
- Published
- 2026-02-05
- DOI
- https://doi.org/10.1021/jacs.5c21246
- Primary Topic
- Advanced battery technologies research
- Type
- article
- Field-Weighted Citation Impact
- 0.00