Nondipole Effects on Electron Correlation Dynamics of Xe Atoms in Circularly Polarized Laser Fields

We present a joint experimental and theoretical investigation of nondipole effects in strong-field double ionization of xenon atoms driven by circularly polarized 800 nm laser fields. We observe that the Xe^{2+} ion momentum distribution in the laser polarization plane is Gaussian. The correlated two-electron momentum distribution along a specific direction in the polarization plane reveals a distinct four-lobe structure. We also measure the photoelectron momentum shift of double ionization along the laser propagation direction, which is associated with the nondipole effect. We find that the nondipole effect shows a remarkable enhancement in momentum shift for low-energy electrons, which deviates from the expectation within the picture of sequential double ionization. We develop a nondipole-corrected two-electron classical trajectory Monte Carlo (CTMC) model that reproduces the experimental observations. The abnormal momentum shift of low-energy electrons originates from recollision-induced linear momentum redistribution. Furthermore, the sensitivity of the nondipole effect to the recollision allows us to resolve distinct angular emission patterns between sequential and nonsequential double ionization. These results indicate that the nondipole effect plays a prominent role in electron correlation, and they offer new insights into many-body linear momentum transfer in intense laser-matter interactions.

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Publication Details

Journal
Physical Review Letters
Published
2026-01-30
DOI
https://doi.org/10.1103/55pk-rxzg
Primary Topic
Laser-Matter Interactions and Applications
Type
article
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article

Nondipole Effects on Electron Correlation Dynamics of Xe Atoms in Circularly Polarized Laser Fields

Qihuang Gong, Y. Liu, YongKai DENG, Chengyin Wu et al.
Physical Review Letters
Laser-Matter Interactions and Applications
article

Nondipole Effects on Electron Correlation Dynamics of Xe Atoms in Circularly Polarized Laser Fields

Qihuang Gong, Y. Liu, YongKai DENG, Chengyin Wu, Peipei Ge, Peizeng Li, Xiaoxiao Long, Anonymous
article en

Abstract

We present a joint experimental and theoretical investigation of nondipole effects in strong-field double ionization of xenon atoms driven by circularly polarized 800 nm laser fields. We observe that the Xe^{2+} ion momentum distribution in the laser polarization plane is Gaussian. The correlated two-electron momentum distribution along a specific direction in the polarization plane reveals a distinct four-lobe structure. We also measure the photoelectron momentum shift of double ionization along the laser propagation direction, which is associated with the nondipole effect. We find that the nondipole effect shows a remarkable enhancement in momentum shift for low-energy electrons, which deviates from the expectation within the picture of sequential double ionization. We develop a nondipole-corrected two-electron classical trajectory Monte Carlo (CTMC) model that reproduces the experimental observations. The abnormal momentum shift of low-energy electrons originates from recollision-induced linear momentum redistribution. Furthermore, the sensitivity of the nondipole effect to the recollision allows us to resolve distinct angular emission patterns between sequential and nonsequential double ionization. These results indicate that the nondipole effect plays a prominent role in electron correlation, and they offer new insights into many-body linear momentum transfer in intense laser-matter interactions.

Physical Review LettersVol. 136(7)
King University (US), Peking University (CN), Shanxi University of Traditional Chinese Medicine (CN), Huazhong University of Science and Technology (CN)
Openalex Percentile: Top 70%
Laser-Matter Interactions and Applications
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