Ferromagnetic Ordering in Rashba Superconductive LaAl <sub>0.7</sub> Mn <sub>0.3</sub> O <sub>3</sub> /SrTiO <sub>3</sub> Interface

The combination of ferromagnetism, superconductivity, and spin-orbit coupling in interfacial two-dimensional electron liquids (2DELs) assembles the essential ingredients for realizing tantalized topological or spin polarized superconductivity for interfacial oxitronics. Unfortunately, these ingredients usually compete and are sometimes mutually exclusive. Here, by optimally designing a ferromagnet/superconductor heterostructure (LaAl<sub>0.7</sub>Mn<sub>0.3</sub>O<sub>3</sub>/SrTiO<sub>3</sub>), we demonstrate a ferromagnetic 2DEL with strong Rashba spin-orbit coupling and typical superconducting behavior. More excitingly, Rashba spin-orbit coupling and ferromagnetic order were found to coexist according to the observation of weak antilocalization and butterfly shaped magnetoresistance with clear hysteresis during the superconducting transition. Our revealed coexistence of ferromagnetism, superconductivity, and spin-orbit coupling at the oxide interface provides a fruitful platform to investigate nontrivial properties of spin-polarized supercurrent/topological superconductors and to cultivate applications for superconducting spintronics/quantum computation.

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Publication Details

Journal
ACS Nano
Published
2026-01-28
DOI
https://doi.org/10.1021/acsnano.5c17832
Primary Topic
Electronic and Structural Properties of Oxides
Type
article
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article

Ferromagnetic Ordering in Rashba Superconductive LaAl 0.7 Mn 0.3 O 3 /SrTiO 3 Interface

Hong Ding, Philippe Ohresser, Wen Xiao, Li Lü et al.
ACS Nano
Electronic and Structural Properties of Oxides
article

Ferromagnetic Ordering in Rashba Superconductive LaAl 0.7 Mn 0.3 O 3 /SrTiO 3 Interface

Hong Ding, Philippe Ohresser, Wen Xiao, Li Lü, Yuhao Hong, Zhaoliang Liao, Yulin Gan, Shilin Hu, Lei Wang, Qinghua Zhang, Kai Chen, Guang Yang, Jie Shen
article en

Abstract

The combination of ferromagnetism, superconductivity, and spin-orbit coupling in interfacial two-dimensional electron liquids (2DELs) assembles the essential ingredients for realizing tantalized topological or spin polarized superconductivity for interfacial oxitronics. Unfortunately, these ingredients usually compete and are sometimes mutually exclusive. Here, by optimally designing a ferromagnet/superconductor heterostructure (LaAl<sub>0.7</sub>Mn<sub>0.3</sub>O<sub>3</sub>/SrTiO<sub>3</sub>), we demonstrate a ferromagnetic 2DEL with strong Rashba spin-orbit coupling and typical superconducting behavior. More excitingly, Rashba spin-orbit coupling and ferromagnetic order were found to coexist according to the observation of weak antilocalization and butterfly shaped magnetoresistance with clear hysteresis during the superconducting transition. Our revealed coexistence of ferromagnetism, superconductivity, and spin-orbit coupling at the oxide interface provides a fruitful platform to investigate nontrivial properties of spin-polarized supercurrent/topological superconductors and to cultivate applications for superconducting spintronics/quantum computation.

ACS NanoVol. 20(5)
University of Science and Technology of China (CN), Shanghai Jiao Tong University (CN), Chinese Academy of Sciences (CN), Synchrotron soleil (FR), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), Yukhnovskii Institute for Condensed Matter Physics of the National Academy of Sciences of Ukraine (UA), National Synchrotron Radiation Laboratory (CN)
Openalex Percentile: Top 75%
Electronic and Structural Properties of Oxides
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