Synthesis, Physicochemical Properties, and Computational Analysis of Tris(fluoromethyl)Alkyl Building Blocks
A concise and scalable synthesis of tris(fluoromethyl)alkyl-building blocks (including amines, carboxylic acids, alcohols, and bromides) starting from commercially available 3,3-bis(bromomethyl)oxetane is reported. Comprehensive physicochemical profiling of the corresponding amines and carboxylic acids (by measuring their pK<sub>a</sub> and LogP values), benchmarked against less fluorinated and nonfluorinated counterparts, showed that the tris(fluoromethyl)methyl (β,β',β''-trifluro-tert-butyl, (FCH<sub>2</sub>)<sub>3</sub>C, TFTB) group mimics the electronic and polarity-modulating properties of CF<sub>3</sub> and CF<sub>3</sub>CH<sub>2</sub> substituents despite substantially larger steric volume. Conformational analysis shows that the (FCH<sub>2</sub>)<sub>3</sub>C group adopts a restricted set of low-energy conformations governed by through-space electrostatic interactions, with C═O···H─C and C─F···H─C contacts playing a crucial stabilizing role. Molecular electrostatic potential analysis rationalizes both the anomalous lipophilicity trends and the CF<sub>3</sub>-like polarity modulation of this group. Together, these data confirm the TFTB group as a valuable motif for isosteric replacement in drug design.
Authors
- Yurii Pustovit
- Oleksandr O. Grygorenko (ORCID: https://orcid.org/0000-0002-6036-5859)
- Oleksandr P. Blahun (ORCID: https://orcid.org/0000-0002-3857-2878)
- Mykhailo O. Redka
- Anton V. Chernykh (ORCID: https://orcid.org/0000-0002-2292-4138)
- Dmytro Lesyk (ORCID: https://orcid.org/0009-0001-3391-5165)
- Alina T. Bezuhla
- Oleksandr S. Liashuk
- Petro Borysko
- Denys Klyukovskyi
Institutions
- Taras Shevchenko National University of Kyiv (UA)
- Institute of Bioorganic Chemistry and Petrochemistry V.P. Kukhar (UA)
- Institute of Organic Chemistry (UA)
- Enamine (Ukraine) (UA)
- V. N. Karazin Kharkiv National University (UA)
Publication Details
- Journal
- Chemistry - A European Journal
- Published
- 2026-01-28
- DOI
- https://doi.org/10.1002/chem.70736
- Primary Topic
- Fluorine in Organic Chemistry
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Ministry of Education and Science of Ukraine
- Enamine