Tunable superconductivity coexisting with the anomalous Hall effect in a transition metal dichalcogenide

Transition metal dichalcogenides display a high technological potential due to their wide range of electronic ground states. Here, we unveil that by tuning hydrostatic pressure P, a cascade of electronic phase transitions can be induced in the few-layer transition metal dichalcogenide 1T'-WS. As P increases, we observe the suppression of superconductivity with the concomitant emergence of an anomalous Hall effect (AHE) at GPa. Above 1.6GPa, we uncover a reentrant superconducting state emerging from a state still exhibiting AHE. This superconducting state competes with the AHE state and shows a marked increase in superconducting anisotropy with respect to the ambient pressure phase, suggesting a distinct pairing symmetry. We demonstrate that 1T'-WS concomitantly transitions into a strong topological phase with different band orbital characters and Fermi surfaces contributing to the superconductivity. These findings position 1T'-WS as a tunable superconductor, wherein superconductivity, AHE, and band features can be tuned reversibly.

Publication Details

Journal
Universität Zürich, ZORA
Published
2025-03-10
DOI
https://doi.org/10.5167/uzh-283571
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
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article

Tunable superconductivity coexisting with the anomalous Hall effect in a transition metal dichalcogenide

Universität Zürich, ZORA
2D Materials and Applications
article

Tunable superconductivity coexisting with the anomalous Hall effect in a transition metal dichalcogenide

article en

Abstract

Transition metal dichalcogenides display a high technological potential due to their wide range of electronic ground states. Here, we unveil that by tuning hydrostatic pressure P, a cascade of electronic phase transitions can be induced in the few-layer transition metal dichalcogenide 1T'-WS. As P increases, we observe the suppression of superconductivity with the concomitant emergence of an anomalous Hall effect (AHE) at GPa. Above 1.6GPa, we uncover a reentrant superconducting state emerging from a state still exhibiting AHE. This superconducting state competes with the AHE state and shows a marked increase in superconducting anisotropy with respect to the ambient pressure phase, suggesting a distinct pairing symmetry. We demonstrate that 1T'-WS concomitantly transitions into a strong topological phase with different band orbital characters and Fermi surfaces contributing to the superconductivity. These findings position 1T'-WS as a tunable superconductor, wherein superconductivity, AHE, and band features can be tuned reversibly.

Universität Zürich, ZORA
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Tunable superconductivity coexisting with the anomalous Hall effect in a transition metal dichalcogenide · Universität Zürich, ZORA (2025) | TGRS Research Map | TGRS