Disorder-induced stress–flow misalignment in soft glassy materials revealed using multidirectional shear

Controlling the mechanical response of soft glassy materials-such as emulsions, foams, and colloidal suspensions-is key for many industrial processes. While their steady-state flow behavior is reasonably well understood, their response to complex flow histories, as encountered in operations like pumping or mixing, remains poorly known. Using a custom multiaxis shear apparatus that enables arbitrary changes in flow direction, we investigate how shear history influences the mechanical behavior of a model soft glassy system. We uncover a transient shear response orthogonal to the applied shear direction, together with an anisotropic yield surface. These effects point to an underlying anisotropic distribution of internal stresses imprinted by previous deformation. To rationalize this behavior, we use a mesoscopic elastoplastic model, demonstrating that local mechanical disorder governs the emergence of macroscopic stress-flow misalignment. Our findings offer a route to experimentally probe the distribution of local yield stresses in soft glassy materials.

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Publication Details

Journal
Proceedings of the National Academy of Sciences
Published
2026-01-22
DOI
https://doi.org/10.1073/pnas.2521603123
Primary Topic
Material Dynamics and Properties
Type
article
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article

Disorder-induced stress–flow misalignment in soft glassy materials revealed using multidirectional shear

Proceedings of the National Academy of Sciences
Material Dynamics and Properties
article

Disorder-induced stress–flow misalignment in soft glassy materials revealed using multidirectional shear

article en

Abstract

Controlling the mechanical response of soft glassy materials-such as emulsions, foams, and colloidal suspensions-is key for many industrial processes. While their steady-state flow behavior is reasonably well understood, their response to complex flow histories, as encountered in operations like pumping or mixing, remains poorly known. Using a custom multiaxis shear apparatus that enables arbitrary changes in flow direction, we investigate how shear history influences the mechanical behavior of a model soft glassy system. We uncover a transient shear response orthogonal to the applied shear direction, together with an anisotropic yield surface. These effects point to an underlying anisotropic distribution of internal stresses imprinted by previous deformation. To rationalize this behavior, we use a mesoscopic elastoplastic model, demonstrating that local mechanical disorder governs the emergence of macroscopic stress-flow misalignment. Our findings offer a route to experimentally probe the distribution of local yield stresses in soft glassy materials.

Proceedings of the National Academy of SciencesVol. 123(4)
Centre National de la Recherche Scientifique (FR), Université de Bordeaux (FR), Institut za filozofiju (HR), Observatoire de la Côte d’Azur (FR), Institut de Physique de Nice (FR), Université Grenoble Alpes (FR)
Openalex Percentile: Top 80%
Material Dynamics and Properties
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Disorder-induced stress–flow misalignment in soft glassy materials revealed using multidirectional shear · Proceedings of the National Academy of Sciences (2026) | TGRS Research Map | TGRS