Radiopurity assay of archaeological lead and related compounds for astroparticle physics by mass spectrometry and gamma-ray spectrometry

A novel and rapid method is introduced for determining thorium (Th) and uranium (U) concentrations in archaeological lead and related compounds to be used in astroparticle physic. This method involves chromatographic pre-concentration and inductively coupled plasma mass spectrometry (ICP-MS). Combined data from mass spectrometry and gamma-ray spectrometry measurements are presented. Excellent results were achieved in terms of reliability and sensitivity (ngˑkg<sup>-1</sup>), even without introducing Th and U isotopes as tracers.

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Publication Details

Journal
Applied Radiation and Isotopes
Published
2026-01-21
DOI
https://doi.org/10.1016/j.apradiso.2026.112458
Primary Topic
Radioactive contamination and transfer
Type
article
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article

Radiopurity assay of archaeological lead and related compounds for astroparticle physics by mass spectrometry and gamma-ray spectrometry

L. Pagnanini, Federico Filippini, Luigi Cappelli, M. Clemenza et al.
Applied Radiation and Isotopes
Radioactive contamination and transfer
article

Radiopurity assay of archaeological lead and related compounds for astroparticle physics by mass spectrometry and gamma-ray spectrometry

L. Pagnanini, Federico Filippini, Luigi Cappelli, M. Clemenza, Stefano Nisi, Matthias Laubenstein, Luca Pattavina
article en

Abstract

A novel and rapid method is introduced for determining thorium (Th) and uranium (U) concentrations in archaeological lead and related compounds to be used in astroparticle physic. This method involves chromatographic pre-concentration and inductively coupled plasma mass spectrometry (ICP-MS). Combined data from mass spectrometry and gamma-ray spectrometry measurements are presented. Excellent results were achieved in terms of reliability and sensitivity (ngˑkg<sup>-1</sup>), even without introducing Th and U isotopes as tracers.

Applied Radiation and IsotopesVol. 230
Istituto Nazionale di Fisica Nucleare, Laboratori Nazionali del Gran Sasso (IT), Istituto Nazionale di Fisica Nucleare, Sezione di Milano Bicocca (IT), Gran Sasso Science Institute (IT), University of Milano-Bicocca (IT)
Openalex Percentile: Top 88%
Radioactive contamination and transfer
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Radiopurity assay of archaeological lead and related compounds for astroparticle physics by mass spectrometry and gamma-ray spectrometry — L. Pagnanini, Federico Filippini, et al. · Applied Radiation and Isotopes (2026) | TGRS Research Map | TGRS