Magnetic field tuned magnetic order and metamagnetic criticality in nonstoichiometric <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>CeAuBi</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

We present a detailed study of magnetization, resistivity, heat capacity, and X-ray and neutron powder diffraction measurements performed on single crystals of non-stoichiometric CeAuBi$_2$, Au deficiency 18$\%$, a strongly correlated antiferromagnet with Néel temperature T$_N$ = 13.2 K. Field-dependent magnetization measurements reveal a large magnetic anisotropy at low temperatures with an easy axis along the crystallographic c-axis, in which direction a spin-flop transition exhibits strong features in magnetization, specific heat, and resistivity at H$_c$ = 75 kOe. The constructed temperature-field phase diagram connects this transition to the suppression of magnetic order, which evolves from a second-order nature into a first-order transition that bifurcates at the spin-flop into three transitions below 1 K. The smoothed nature of the metamagnetic transitions in non-stoichiometric CeAuBi$_2$ is well described by an Ising model with weak quenched disorder, suggesting that the presence of Au vacancies is sufficient to smear the complex metamagnetic behavior and tune the critical behavior of magnetic order.

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Journal
Physical review. B./Physical review. B
Published
2026-01-15
DOI
https://doi.org/10.1103/1qcc-by7y
Primary Topic
Rare-earth and actinide compounds
Type
article
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Magnetic field tuned magnetic order and metamagnetic criticality in nonstoichiometric <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>CeAuBi</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

Chris Eckberg, K Wang, Tristin Metz, David Graf et al.
Physical review. B./Physical review. B
Rare-earth and actinide compounds
article

Magnetic field tuned magnetic order and metamagnetic criticality in nonstoichiometric <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>CeAuBi</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>

Chris Eckberg, K Wang, Tristin Metz, David Graf, J. Paglione, Yasuyuki Nakajima, Thomas Vojta, Hyunsoo Kim, Anonymous, Nicholas P. Butch, Shanta R. Saha, Jie Yong
article en

Abstract

We present a detailed study of magnetization, resistivity, heat capacity, and X-ray and neutron powder diffraction measurements performed on single crystals of non-stoichiometric CeAuBi$_2$, Au deficiency 18$\%$, a strongly correlated antiferromagnet with Néel temperature T$_N$ = 13.2 K. Field-dependent magnetization measurements reveal a large magnetic anisotropy at low temperatures with an easy axis along the crystallographic c-axis, in which direction a spin-flop transition exhibits strong features in magnetization, specific heat, and resistivity at H$_c$ = 75 kOe. The constructed temperature-field phase diagram connects this transition to the suppression of magnetic order, which evolves from a second-order nature into a first-order transition that bifurcates at the spin-flop into three transitions below 1 K. The smoothed nature of the metamagnetic transitions in non-stoichiometric CeAuBi$_2$ is well described by an Ising model with weak quenched disorder, suggesting that the presence of Au vacancies is sufficient to smear the complex metamagnetic behavior and tune the critical behavior of magnetic order.

Physical review. B./Physical review. BVol. 113(5)
Florida State University (US), Canadian Institute for Advanced Research (CA), National Institute of Standards and Technology (US), Missouri University of Science and Technology (US), National Institute of Standards (EG), University of Maryland, College Park (US)
Openalex Percentile: Top 82%
Rare-earth and actinide compounds
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