Giant THz Magnetoresistance and Refractive Index Shift in Spin-Textured EuTe <sub>2</sub> via Field-Controlled Bandgap
The realization of terahertz (THz)-frequency magneto effects presents a fundamental challenge and opportunity for ultrafast spintronics. Herein, we demonstrate record-breaking THz giant magnetoresistance (GMR) and anisotropic magnetoresistance (AMR) in EuTe<sub>2</sub>, a model noncollinear antiferromagnet. Under a 2.5 T magnetic field, the THz GMR exceeds 90%, while the THz AMR reaches an unprecedented 450% at 0.48 THz (2 T) and 5 K, surpassing known MR effects in this frequency regime. Further, THz absorption spectroscopy provides the first direct optical evidence of spin-texture bands via a field-induced bandgap reconstruction from 4.9 to 2.2 meV, linking the THz GMR/AMR to spin-orientation control rather than conventional spin arrangement manipulation. Moreover, a pronounced refractive index shift (Δ<i>n</i> ∼ 0.8) results from magnetic field-induced bandgap closure and permeability tuning, a mechanism unlike thermal effects. Our findings promote spin-texture materials as a promising platform for high-frequency spintronics and magneto-optics, while also establishing THz spectroscopy as a transformative tool for probing quantum dynamics.
Authors
- Z Sheng
- Zhuang Ren (ORCID: https://orcid.org/0000-0002-8470-8211)
- Zhian Xu (ORCID: https://orcid.org/0000-0002-2748-0046)
- Xiao Chang (ORCID: https://orcid.org/0009-0006-5103-531X)
- Z. C. Zhong
- Pengli Hao
- Biwen Huang
- Yanfeng Guo
- Xinyu Liu
Institutions
- University of Science and Technology of China (CN)
- Chinese Academy of Sciences (CN)
- ShanghaiTech University (CN)
- High Magnetic Field Laboratory (CN)
- VPIphotonics (Germany) (DE)
- Collaborative Innovation Center of Advanced Microstructures (CN)
- Quantum Technologies (Sweden) (SE)
- Taiyuan University of Science and Technology (CN)
- Nanjing University (CN)
Publication Details
- Journal
- ACS Applied Materials & Interfaces
- Published
- 2026-01-14
- DOI
- https://doi.org/10.1021/acsami.5c20467
- Primary Topic
- Topological Materials and Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 0.00