Giant THz Magnetoresistance and Refractive Index Shift in Spin-Textured EuTe <sub>2</sub> via Field-Controlled Bandgap

The realization of terahertz (THz)-frequency magneto effects presents a fundamental challenge and opportunity for ultrafast spintronics. Herein, we demonstrate record-breaking THz giant magnetoresistance (GMR) and anisotropic magnetoresistance (AMR) in EuTe<sub>2</sub>, a model noncollinear antiferromagnet. Under a 2.5 T magnetic field, the THz GMR exceeds 90%, while the THz AMR reaches an unprecedented 450% at 0.48 THz (2 T) and 5 K, surpassing known MR effects in this frequency regime. Further, THz absorption spectroscopy provides the first direct optical evidence of spin-texture bands via a field-induced bandgap reconstruction from 4.9 to 2.2 meV, linking the THz GMR/AMR to spin-orientation control rather than conventional spin arrangement manipulation. Moreover, a pronounced refractive index shift (Δ<i>n</i> ∼ 0.8) results from magnetic field-induced bandgap closure and permeability tuning, a mechanism unlike thermal effects. Our findings promote spin-texture materials as a promising platform for high-frequency spintronics and magneto-optics, while also establishing THz spectroscopy as a transformative tool for probing quantum dynamics.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2026-01-14
DOI
https://doi.org/10.1021/acsami.5c20467
Primary Topic
Topological Materials and Phenomena
Type
article
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article

Giant THz Magnetoresistance and Refractive Index Shift in Spin-Textured EuTe 2 via Field-Controlled Bandgap

Z Sheng, Zhuang Ren, Zhian Xu, Xiao Chang et al.
ACS Applied Materials & Interfaces
Topological Materials and Phenomena
article

Giant THz Magnetoresistance and Refractive Index Shift in Spin-Textured EuTe 2 via Field-Controlled Bandgap

Z Sheng, Zhuang Ren, Zhian Xu, Xiao Chang, Z. C. Zhong, Pengli Hao, Biwen Huang, Yanfeng Guo, Xinyu Liu
article en

Abstract

The realization of terahertz (THz)-frequency magneto effects presents a fundamental challenge and opportunity for ultrafast spintronics. Herein, we demonstrate record-breaking THz giant magnetoresistance (GMR) and anisotropic magnetoresistance (AMR) in EuTe<sub>2</sub>, a model noncollinear antiferromagnet. Under a 2.5 T magnetic field, the THz GMR exceeds 90%, while the THz AMR reaches an unprecedented 450% at 0.48 THz (2 T) and 5 K, surpassing known MR effects in this frequency regime. Further, THz absorption spectroscopy provides the first direct optical evidence of spin-texture bands via a field-induced bandgap reconstruction from 4.9 to 2.2 meV, linking the THz GMR/AMR to spin-orientation control rather than conventional spin arrangement manipulation. Moreover, a pronounced refractive index shift (Δ<i>n</i> ∼ 0.8) results from magnetic field-induced bandgap closure and permeability tuning, a mechanism unlike thermal effects. Our findings promote spin-texture materials as a promising platform for high-frequency spintronics and magneto-optics, while also establishing THz spectroscopy as a transformative tool for probing quantum dynamics.

ACS Applied Materials & InterfacesVol. 18(3)
University of Science and Technology of China (CN), Chinese Academy of Sciences (CN), ShanghaiTech University (CN), High Magnetic Field Laboratory (CN), VPIphotonics (Germany) (DE), Collaborative Innovation Center of Advanced Microstructures (CN), Quantum Technologies (Sweden) (SE), Taiyuan University of Science and Technology (CN), Nanjing University (CN)
Openalex Percentile: Top 85%
Topological Materials and Phenomena
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Giant THz Magnetoresistance and Refractive Index Shift in Spin-Textured EuTe <sub>2</sub> via Field-Controlled Bandgap — Z Sheng, Zhuang Ren, et al. · ACS Applied Materials & Interfaces (2026) | TGRS Research Map | TGRS