Use of solid fat-tailored oleogels loaded with α-tocopherol as fat replacers to improve the nutritional profile of cookies

Introduction Oleogels containing low candelilla wax (CLW) content (<2.5%) loaded with α-tocopherol mimic the rheological properties of butter, margarine, and partially hydrogenated fat. However, their use in food to enhance vitamin E intake remains unexplored. This study investigated CLW-based oleogels loaded with α-tocopherol, developed previously to replicate the rheological properties of butter ( O btr ), margarine ( O mgn ), and partially hydrogenated fat ( O hgf ), as full replacements for these fats in cookies. Methods Doughs and cookies containing O btr , O mgn , or O hgf were assessed for instrumental color, rheological, textural, and baking properties. Principal component analysis (PCA) was applied to investigate the clustering and similarities between oleogel-based samples and their respective reference solid fats. Results Doughs with oleogels exhibited a darker surface and a weaker structure compared to those with solid fats. Cookies with oleogels were darker, softer, and less crispy than those made with solid fats. Cookies with O MGN exhibited a spread factor comparable to that of margarine, although other dimensional and textural parameters differed. PCA revealed no distinct clustering between the doughs containing oleogels and those with their respective solid fats (PC1 = 56.1%; PC2 = 28.9%). However, cookies containing oleogels clustered closely with those with partially hydrogenated fat (PC1 = 58.1%; PC2 = 38.8%), suggesting that reproducing the functional response of partially hydrogenated fat is more feasible than that of butter or margarine. Results Therefore, oleogels with low CLW content loaded with α-tocopherol present a promising alternative for replacing hydrogenated fats in cookies formulations.

Authors

Institutions

Publication Details

Journal
Frontiers in Soft Matter
Published
2026-01-12
DOI
https://doi.org/10.3389/frsfm.2025.1741918
Primary Topic
Food Chemistry and Fat Analysis
Type
article
Field-Weighted Citation Impact
0.00

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Use of solid fat-tailored oleogels loaded with α-tocopherol as fat replacers to improve the nutritional profile of cookies

Gabriela Baptista Brito, Carlos Adam Conte‐Júnior, M Nele, Thiago O. Marinho et al.
Frontiers in Soft Matter
Food Chemistry and Fat Analysis
article

Use of solid fat-tailored oleogels loaded with α-tocopherol as fat replacers to improve the nutritional profile of cookies

Gabriela Baptista Brito, Carlos Adam Conte‐Júnior, M Nele, Thiago O. Marinho, Alexandre Guedes Torres, Vanessa Oliveira Di Sarli Peixoto, Vanessa Naciuk Castelo-Branco
article en

Abstract

Introduction Oleogels containing low candelilla wax (CLW) content (<2.5%) loaded with α-tocopherol mimic the rheological properties of butter, margarine, and partially hydrogenated fat. However, their use in food to enhance vitamin E intake remains unexplored. This study investigated CLW-based oleogels loaded with α-tocopherol, developed previously to replicate the rheological properties of butter ( O btr ), margarine ( O mgn ), and partially hydrogenated fat ( O hgf ), as full replacements for these fats in cookies. Methods Doughs and cookies containing O btr , O mgn , or O hgf were assessed for instrumental color, rheological, textural, and baking properties. Principal component analysis (PCA) was applied to investigate the clustering and similarities between oleogel-based samples and their respective reference solid fats. Results Doughs with oleogels exhibited a darker surface and a weaker structure compared to those with solid fats. Cookies with oleogels were darker, softer, and less crispy than those made with solid fats. Cookies with O MGN exhibited a spread factor comparable to that of margarine, although other dimensional and textural parameters differed. PCA revealed no distinct clustering between the doughs containing oleogels and those with their respective solid fats (PC1 = 56.1%; PC2 = 28.9%). However, cookies containing oleogels clustered closely with those with partially hydrogenated fat (PC1 = 58.1%; PC2 = 38.8%), suggesting that reproducing the functional response of partially hydrogenated fat is more feasible than that of butter or margarine. Results Therefore, oleogels with low CLW content loaded with α-tocopherol present a promising alternative for replacing hydrogenated fats in cookies formulations.

Frontiers in Soft MatterVol. 5
Universidade Federal do Rio de Janeiro (BR)
Coordenação de Aperfeiçoamento de Pessoal de Nível Superior, Conselho Nacional de Desenvolvimento Científico e Tecnológico, Fundação Carlos Chagas Filho de Amparo à Pesquisa do Estado do Rio de Janeiro
Zero hunger
Openalex Percentile: Top 91%
Food Chemistry and Fat Analysis
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.