Cavity Controls Core-to-Core Resonant Inelastic X-Ray Scattering
X-ray cavity quantum optics with inner-shell transitions has been limited by the spectral overlap between resonant and continuum states. Here, we report the first experimental demonstration of cavity-controlled core-to-core resonant inelastic x-ray scattering (RIXS). We suppress the absorption-edge effects by monitoring the RIXS profile, thereby resolving the resonant state from the overlapping continuum. We observe distinct cavity-induced energy shifts and cavity-enhanced decay rates in the 2p3d RIXS spectra of WSi_{2}. These effects, manifesting as stretched or shifted profiles in the RIXS planes, enable novel spectroscopic applications via cavity-controlled core-hole states. Our results establish core-to-core RIXS as a powerful tool to manipulate inner-shell dynamics in x-ray cavities, offering new avenues for integrating quantum optical effects with x-ray spectroscopy.
Authors
- J.-P Rueff
- W. B. Li
- T. P. Li
- L-F Zhu
- T. Hu
- Z-Q Zhao
- Anonymous
- A. Khadiev
- F. Alves Lima
- B.-H. Wang
- X.-Y. Wang
- H.-C. Wang
- Y. Uemura
- Y. Su
- O. J. L. Fox
- J. M. Ablett
Institutions
- Tongji University (CN)
- University of Science and Technology of China (CN)
- GSI Helmholtz Centre for Heavy Ion Research (DE)
- Synchrotron soleil (FR)
- Deutsches Elektronen-Synchrotron DESY (DE)
- Diamond Light Source (GB)
- Sorbonne Université (FR)
- Laboratoire de Chimie Physique - Matière et Rayonnement (FR)
- Laboratoire Médiations (FR)
- European X-Ray Free-Electron Laser (DE)
Publication Details
- Journal
- Physical Review Letters
- Published
- 2026-01-09
- DOI
- https://doi.org/10.1103/z6xz-p7cm
- Primary Topic
- Crystallography and Radiation Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 0.00