(Ir)Relevance of Disorder for Superconductivity in Cuprates

In cuprates that exhibit high-temperature superconductivity (HTS), as the doping level p is increased beyond the optimal value, the superfluid density n_{s0} decreases and eventually vanishes, closely tracking the critical temperature T_{c}. This has been interpreted using a dirty-d-wave extension of the Bardeen-Cooper-Schrieffer theory, assuming that T_{c} and n_{s0} decrease with increasing disorder and pair breaking. To test this hypothesis, we tuned the doping level in overdoped La_{2-x}Sr_{x}CuO_{4-δ} films by electrolyte gating, measured several parameters used to quantify the level of disorder (the residual resistivity ratio RRR, the mean free path l_{0}, and the electron mobility μ), and studied how T_{c} and n_{s0} scale with these. The experimentally measured dependence turned out to be the opposite of the expected-T_{c} and n_{s0} increased with increasing disorder. This brings the question of the true origin of the demise of T_{c} and n_{s0} with overdoping back to the center stage of the quest to decipher the HTS enigma.

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Publication Details

Journal
Physical Review Letters
Published
2026-01-08
DOI
https://doi.org/10.1103/5nzl-fjmx
Primary Topic
Physics of Superconductivity and Magnetism
Type
article
Field-Weighted Citation Impact
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article

(Ir)Relevance of Disorder for Superconductivity in Cuprates

I. Božović, Xu-Gang He, Anonymous, A. T. Bollinger
Physical Review Letters
Physics of Superconductivity and Magnetism
article

(Ir)Relevance of Disorder for Superconductivity in Cuprates

I. Božović, Xu-Gang He, Anonymous, A. T. Bollinger
article en

Abstract

In cuprates that exhibit high-temperature superconductivity (HTS), as the doping level p is increased beyond the optimal value, the superfluid density n_{s0} decreases and eventually vanishes, closely tracking the critical temperature T_{c}. This has been interpreted using a dirty-d-wave extension of the Bardeen-Cooper-Schrieffer theory, assuming that T_{c} and n_{s0} decrease with increasing disorder and pair breaking. To test this hypothesis, we tuned the doping level in overdoped La_{2-x}Sr_{x}CuO_{4-δ} films by electrolyte gating, measured several parameters used to quantify the level of disorder (the residual resistivity ratio RRR, the mean free path l_{0}, and the electron mobility μ), and studied how T_{c} and n_{s0} scale with these. The experimentally measured dependence turned out to be the opposite of the expected-T_{c} and n_{s0} increased with increasing disorder. This brings the question of the true origin of the demise of T_{c} and n_{s0} with overdoping back to the center stage of the quest to decipher the HTS enigma.

Physical Review LettersVol. 136(7)
Brookhaven National Laboratory (US), Yale University (US), Physical Sciences (United States) (US)
Openalex Percentile: Top 89%
Physics of Superconductivity and Magnetism
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