Intensity-dependent interferences in strong-field Rydberg-state excitation

We conduct a systematic investigation of the oscillations of the Rydberg-state populations as a function of intensity arising from strong-field multiphoton excitation of Rydberg atoms. By numerically solving the time-dependent Schrödinger equation and by constructing a quantum model based on Freeman resonances, we elucidate the underlying physical mechanisms governing the intensity-dependent oscillatory behavior of the Rydberg-state population dynamics. Our analysis shows that these oscillations originate from the synergistic interplay of three distinct quantum-interference mechanisms: (1) interference between excitation pathways at the rising and falling edges of the laser pulse (long-time interference), (2) interference between different optical cycles within the same side of the laser pulse (short-time interference), and (3) interference within individual optical cycles (intracycle interference). Additionally, we find that ground-state depletion has varying degrees of influence on the oscillation patterns formed by the three interference mechanisms under different laser-intensity conditions.

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Publication Details

Journal
Physical Review Research
Published
2026-01-08
DOI
https://doi.org/10.1103/4d6p-55n1
Primary Topic
Laser-Matter Interactions and Applications
Type
article
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article

Intensity-dependent interferences in strong-field Rydberg-state excitation

Jing Chen, W B Becker, Li Guo, C. F. Liang et al.
Physical Review Research
Laser-Matter Interactions and Applications
article

Intensity-dependent interferences in strong-field Rydberg-state excitation

Jing Chen, W B Becker, Li Guo, C. F. Liang, Anonymous
article en

Abstract

We conduct a systematic investigation of the oscillations of the Rydberg-state populations as a function of intensity arising from strong-field multiphoton excitation of Rydberg atoms. By numerically solving the time-dependent Schrödinger equation and by constructing a quantum model based on Freeman resonances, we elucidate the underlying physical mechanisms governing the intensity-dependent oscillatory behavior of the Rydberg-state population dynamics. Our analysis shows that these oscillations originate from the synergistic interplay of three distinct quantum-interference mechanisms: (1) interference between excitation pathways at the rising and falling edges of the laser pulse (long-time interference), (2) interference between different optical cycles within the same side of the laser pulse (short-time interference), and (3) interference within individual optical cycles (intracycle interference). Additionally, we find that ground-state depletion has varying degrees of influence on the oscillation patterns formed by the three interference mechanisms under different laser-intensity conditions.

Physical Review ResearchVol. 8(1)
University of Science and Technology of China (CN), Shanghai Normal University (CN), Hefei University (CN), Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE), Institute of Applied Physics and Computational Mathematics (CN)
Openalex Percentile: Top 91%
Laser-Matter Interactions and Applications
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Intensity-dependent interferences in strong-field Rydberg-state excitation — Jing Chen, W B Becker, et al. · Physical Review Research (2026) | TGRS Research Map | TGRS