Intensity-dependent interferences in strong-field Rydberg-state excitation
We conduct a systematic investigation of the oscillations of the Rydberg-state populations as a function of intensity arising from strong-field multiphoton excitation of Rydberg atoms. By numerically solving the time-dependent Schrödinger equation and by constructing a quantum model based on Freeman resonances, we elucidate the underlying physical mechanisms governing the intensity-dependent oscillatory behavior of the Rydberg-state population dynamics. Our analysis shows that these oscillations originate from the synergistic interplay of three distinct quantum-interference mechanisms: (1) interference between excitation pathways at the rising and falling edges of the laser pulse (long-time interference), (2) interference between different optical cycles within the same side of the laser pulse (short-time interference), and (3) interference within individual optical cycles (intracycle interference). Additionally, we find that ground-state depletion has varying degrees of influence on the oscillation patterns formed by the three interference mechanisms under different laser-intensity conditions.
Authors
- Jing Chen (ORCID: https://orcid.org/0000-0003-0538-689X)
- W B Becker
- Li Guo
- C. F. Liang
- Anonymous
Institutions
- University of Science and Technology of China (CN)
- Shanghai Normal University (CN)
- Hefei University (CN)
- Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE)
- Institute of Applied Physics and Computational Mathematics (CN)
Publication Details
- Journal
- Physical Review Research
- Published
- 2026-01-08
- DOI
- https://doi.org/10.1103/4d6p-55n1
- Primary Topic
- Laser-Matter Interactions and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00