Extrinsic and Intrinsic Nonlinear Planar Hall Effect in <i>T</i> <sub>d</sub> -MoTe <sub>2</sub>

<i>T</i><sub>d</sub>-MoTe<sub>2</sub>, a semimetallic material with broken inversion symmetry, allows a rich variety of nonlinear transport phenomena which may manifest intriguing quantum geometry of the band structure. Here, we report the observation of a nonlinear planar Hall effect in <i>T</i><sub>d</sub>-MoTe<sub>2</sub> over a broad temperature range (2 to 150 K). The nonlinear Hall voltage scales quadratically (linearly) with the applied electric (magnetic) field and shows distinct angular dependence on the in-plane magnetic field: a cosine (sine) relationship when the electric field aligns with the <i>a</i> axis (<i>b</i> axis). Combined first-principles calculations and scaling analysis of experimental data reveal two scaling terms, including an intrinsic contribution from Berry connection polarizability of band structure and an extrinsic nonlinear Drude-like contribution. This study not only expands the understanding of nonlinear Hall transport mechanisms in low-symmetry materials but also suggests potential applications in precision magnetic field sensing and electronic devices exploiting directional charge transport.

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Publication Details

Journal
Nano Letters
Published
2026-01-06
DOI
https://doi.org/10.1021/acs.nanolett.5c05007
Primary Topic
Topological Materials and Phenomena
Type
article
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article

Extrinsic and Intrinsic Nonlinear Planar Hall Effect in T d -MoTe 2

Shengyuan A. Yang, Cong Xiao, H. Wang, Naizhou Wang et al.
Nano Letters
Topological Materials and Phenomena
article

Extrinsic and Intrinsic Nonlinear Planar Hall Effect in T d -MoTe 2

Shengyuan A. Yang, Cong Xiao, H. Wang, Naizhou Wang, Haiyang Pan, Liheng An, Yue-Xin Huang, Jingsheng Chen, Weibo Gao, Xueqi Hu
article en

Abstract

<i>T</i><sub>d</sub>-MoTe<sub>2</sub>, a semimetallic material with broken inversion symmetry, allows a rich variety of nonlinear transport phenomena which may manifest intriguing quantum geometry of the band structure. Here, we report the observation of a nonlinear planar Hall effect in <i>T</i><sub>d</sub>-MoTe<sub>2</sub> over a broad temperature range (2 to 150 K). The nonlinear Hall voltage scales quadratically (linearly) with the applied electric (magnetic) field and shows distinct angular dependence on the in-plane magnetic field: a cosine (sine) relationship when the electric field aligns with the <i>a</i> axis (<i>b</i> axis). Combined first-principles calculations and scaling analysis of experimental data reveal two scaling terms, including an intrinsic contribution from Berry connection polarizability of band structure and an extrinsic nonlinear Drude-like contribution. This study not only expands the understanding of nonlinear Hall transport mechanisms in low-symmetry materials but also suggests potential applications in precision magnetic field sensing and electronic devices exploiting directional charge transport.

Nano LettersVol. 26(2)
Centre for Quantum Technologies (SG), Hong Kong Polytechnic University (HK), National University of Singapore (SG), Nanyang Technological University (SG), Hong Kong University of Science and Technology (HK), Fudan University (CN), Center for Theoretical Physics (PL), Westlake University (CN), Quantum Applied Science and Research (United States) (US), Institute for Schools of the Future (US), Institute for the Future (US), Institute for Advanced Study (DE), Institute of Natural Science (KP), Great Bay University
Openalex Percentile: Top 93%
Topological Materials and Phenomena
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