A conveyor-belt magneto-optical trap of CaF

Achieving high-density samples of laser-cooled molecules is a critical step toward advancing applications in precision measurements, ultracold chemistry and quantum science. We report the experimental realization of a high-density conveyor-belt magneto-optical trap for calcium monofluoride (CaF) molecules. The obtained highly-compressed cloud has a mean radius of 64(5) μm and a peak number density of 3.6(5) × 10<sup>10</sup> cm<sup>-3</sup>, a 600-fold increase over the conventional red-detuned MOTs of CaF, and the densest molecular MOT observed to date. Subsequent loading of these molecules into an optical dipole trap yields up to 2.6 × 10<sup>4</sup> trapped molecules at a temperature of 14(2) μK with a peak phase-space density of ~ 2.4 × 10<sup>-6</sup>. This opens new possibilities for a range of applications utilizing high-density, optically trapped ultracold molecules.

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Publication Details

Journal
Nature Communications
Published
2026-01-07
DOI
https://doi.org/10.1038/s41467-025-67944-6
Citations
2
Primary Topic
Cold Atom Physics and Bose-Einstein Condensates
Type
article
Field-Weighted Citation Impact
31.39

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article

A conveyor-belt magneto-optical trap of CaF

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2 citations
Nature Communications
Cold Atom Physics and Bose-Einstein Condensates
31.39
article

A conveyor-belt magneto-optical trap of CaF

Kang-Kuen Ni, Grace K. Li, Christian Hallas, Wolfgang Ketterle, Scarlett S. Yu, John M. Doyle, Yicheng Bao, Loïc Anderegg, Eunmi Chae, Dongkyu Lim, Jiaqi You
article en
2 citations

Abstract

Achieving high-density samples of laser-cooled molecules is a critical step toward advancing applications in precision measurements, ultracold chemistry and quantum science. We report the experimental realization of a high-density conveyor-belt magneto-optical trap for calcium monofluoride (CaF) molecules. The obtained highly-compressed cloud has a mean radius of 64(5) μm and a peak number density of 3.6(5) × 10<sup>10</sup> cm<sup>-3</sup>, a 600-fold increase over the conventional red-detuned MOTs of CaF, and the densest molecular MOT observed to date. Subsequent loading of these molecules into an optical dipole trap yields up to 2.6 × 10<sup>4</sup> trapped molecules at a temperature of 14(2) μK with a peak phase-space density of ~ 2.4 × 10<sup>-6</sup>. This opens new possibilities for a range of applications utilizing high-density, optically trapped ultracold molecules.

Nature CommunicationsVol. 17(1)
University of Southern California (US), Harvard University (US), Korea University (KR), Princeton University (US), Harvard University Press (US), MIT-Harvard Center for Ultracold Atoms (US), Korea University (JP), Massachusetts Institute of Technology (US)
National Science Foundation, U.S. Department of Energy, Office of Science, Multidisciplinary University Research Initiative, Center for Ultracold Atoms, Massachusetts Institute of Technology, Air Force Office of Scientific Research
Openalex Percentile: Top 2%
Cold Atom Physics and Bose-Einstein Condensates
31.39
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