Magnetic properties of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>J</mml:mi> <mml:mtext>eff</mml:mtext> </mml:msub> <mml:mo>=</mml:mo> <mml:mfrac> <mml:mn>1</mml:mn> <mml:mn>2</mml:mn> </mml:mfrac> </m
The subtle interplay between competing degrees of freedom, crystal electric fields, and spin correlations can lead to exotic quantum states in 4f ion-based frustrated triangular lattice antiferromagnets. We present the crystal structure, thermodynamic and muon spin relaxation (μSR) studies of the 4f ion-based frustrated magnet Ba4YbReWO12, wherein Yb3+ ions constitute a triangular lattice. The magnetic susceptibility does not show any signature of spin freezing down to 1.9 K or long-range magnetic ordering down to 0.4 K. The low-temperature Curie-Weiss fit to the inverse magnetic susceptibility data reveals a weak antiferromagnetic exchange interaction, which is corroborated by the fit of magnetic specific heat data following the J1-J2 model with the nearest neighbor exchange interaction of J1 = -0.197 K between the Jeff = 1/2 states of the Yb3+ moments in the lowest Kramers doublet. The lowest Kramers ground state doublet is well separated from the first excited state with a gap of 278 K, as evidenced by our μSR experiments that support the realization of Jeff = 1/2 at low temperatures. The specific heat experiments do not detect a phase transition down to 56 mK. The magnetic specific heat shows a broad maximum 90 mK suggesting a disordered ground state with short range spin correlations. The associated magnetic entropy release at low temperatures is consistent with that expected for the Jeff = 1/2 state. The zero-field μSR measurements show neither the signature of spin freezing nor a phase transition, at least down to 43 mK. Our results suggest a dynamic, disordered ground state in this Jeff = 1/2 frustrated triangular lattice antiferromagnet. Ba4RReWO12 (R=rare earth) offers a viable platform to realize intriguing quantum states borne out of spin-orbit coupling and frustration
Authors
- B. Hitti (ORCID: https://orcid.org/0009-0008-4187-1757)
- J. Khatua (ORCID: https://orcid.org/0000-0003-3562-4131)
- P. Khuntia (ORCID: https://orcid.org/0000-0002-4054-485X)
- Kwang‐Yong Choi (ORCID: https://orcid.org/0000-0001-8213-5395)
- Suyoung Kim (ORCID: https://orcid.org/0000-0001-9212-4913)
- Suheon Lee
- Anonymous
- Eundeok Mun
- Gerald D. Morris
Institutions
- Simon Fraser University (CA)
- Indian Institute of Technology Madras (IN)
- Institute for Basic Science (KR)
- Sungkyunkwan University (KR)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2026-01-06
- DOI
- https://doi.org/10.1103/1fqr-7njx
- Primary Topic
- Advanced Condensed Matter Physics
- Type
- article
- Field-Weighted Citation Impact
- 0.00