Enhanced superconductivity and vortex dynamics in quasi-1D TaS2 nanowires

We report the synthesis of high-quality 2H-TaS2 nanowires via a controlled two-step conversion process from TaS3 precursors, achieving robust superconductivity with a transition temperature Tc ≈ 3.6 K, which is significantly higher than bulk 2H-TaS2 (Tc ≈ 0.8 K). Structural and compositional analyses confirm phase purity and preserved one-dimensional morphology, while magnetotransport measurements reveal an enhanced upper critical field μ0Hc2 (2 K) ≈ 5 T, far exceeding the bulk value (μ0Hc2 (0) ≈ 1.17 T), attributed to dimensional confinement and suppression of charge-density wave order. Magnetic characterization demonstrates complex vortex dynamics, including flux jumps and a second magnetization peak, indicative of strong pinning and crossover from elastic to plastic vortex regimes. These findings establish TaS2 nanowires as a versatile platform for studying superconductivity in reduced dimensions and exploiting confinement-driven quantum phenomena for advanced applications.

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Publication Details

Journal
Applied Physics Letters
Published
2026-01-05
DOI
https://doi.org/10.1063/5.0285670
Primary Topic
2D Materials and Applications
Type
article
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Enhanced superconductivity and vortex dynamics in quasi-1D TaS2 nanowires

Clarissa A. Wisner, Eric W. Bohannan, Mathew Pollard, Visakha Ho et al.
Applied Physics Letters
2D Materials and Applications
article

Enhanced superconductivity and vortex dynamics in quasi-1D TaS2 nanowires

Clarissa A. Wisner, Eric W. Bohannan, Mathew Pollard, Visakha Ho, Yew San Hor
article en

Abstract

We report the synthesis of high-quality 2H-TaS2 nanowires via a controlled two-step conversion process from TaS3 precursors, achieving robust superconductivity with a transition temperature Tc ≈ 3.6 K, which is significantly higher than bulk 2H-TaS2 (Tc ≈ 0.8 K). Structural and compositional analyses confirm phase purity and preserved one-dimensional morphology, while magnetotransport measurements reveal an enhanced upper critical field μ0Hc2 (2 K) ≈ 5 T, far exceeding the bulk value (μ0Hc2 (0) ≈ 1.17 T), attributed to dimensional confinement and suppression of charge-density wave order. Magnetic characterization demonstrates complex vortex dynamics, including flux jumps and a second magnetization peak, indicative of strong pinning and crossover from elastic to plastic vortex regimes. These findings establish TaS2 nanowires as a versatile platform for studying superconductivity in reduced dimensions and exploiting confinement-driven quantum phenomena for advanced applications.

Applied Physics LettersVol. 128(1)
Missouri University of Science and Technology (US)
Openalex Percentile: Top 96%
2D Materials and Applications
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