Convective Onset in Thermal Lensing: Systematic Pulse-Number-Dependent Experiments and Theoretical Insights into the Femtosecond Regime

This study investigates thermal lensing induced by femtosecond-laser pulses, a key technique for examining the thermo-optical response of materials under high-repetition-rate irradiation. Using both experimental and theoretical approaches, this work examines how thermal lensing develops and evolves over time with a focus on the effects of pulse count, pump-on duration, and pump-off duration. The study examines how conduction and convection mechanisms compete during heat dissipation, with conduction dominating at a lower number of pulses. The theoretical approach emphasizes heat generation from single-pulse interactions, which is a central aspect of this research. Importantly, the study also shows the potential thermal lens (TL) amplitude from a single femtosecond pulse, providing insights into the early stages of heat buildup. These results enhance our understanding of heat transfer in ultrafast laser-matter interactions, providing more detailed insight into how thermal lenses form and relax.

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Publication Details

Journal
The Journal of Physical Chemistry B
Published
2026-01-05
DOI
https://doi.org/10.1021/acs.jpcb.5c05468
Primary Topic
Laser Material Processing Techniques
Type
article
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article

Convective Onset in Thermal Lensing: Systematic Pulse-Number-Dependent Experiments and Theoretical Insights into the Femtosecond Regime

Aman Sharma, Debabrata Goswami
The Journal of Physical Chemistry B
Laser Material Processing Techniques
article

Convective Onset in Thermal Lensing: Systematic Pulse-Number-Dependent Experiments and Theoretical Insights into the Femtosecond Regime

Aman Sharma, Debabrata Goswami
article en

Abstract

This study investigates thermal lensing induced by femtosecond-laser pulses, a key technique for examining the thermo-optical response of materials under high-repetition-rate irradiation. Using both experimental and theoretical approaches, this work examines how thermal lensing develops and evolves over time with a focus on the effects of pulse count, pump-on duration, and pump-off duration. The study examines how conduction and convection mechanisms compete during heat dissipation, with conduction dominating at a lower number of pulses. The theoretical approach emphasizes heat generation from single-pulse interactions, which is a central aspect of this research. Importantly, the study also shows the potential thermal lens (TL) amplitude from a single femtosecond pulse, providing insights into the early stages of heat buildup. These results enhance our understanding of heat transfer in ultrafast laser-matter interactions, providing more detailed insight into how thermal lenses form and relax.

The Journal of Physical Chemistry BVol. 130(2)
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Laser Material Processing Techniques
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Convective Onset in Thermal Lensing: Systematic Pulse-Number-Dependent Experiments and Theoretical Insights into the Femtosecond Regime — Aman Sharma, Debabrata Goswami · The Journal of Physical Chemistry B (2026) | TGRS Research Map | TGRS