Investigating the electrical transport properties and electronic structure of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>Zr</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>CuSb</mml:mi> <mml:mn>
The checkerboard lattice has been proposed to host topological flat bands as a result of destructive interference among its various electronic hopping terms. However, it has proven challenging to realize experimentally due to the difficulty of isolating this structure from any significant out-of-plane bonding while maintaining structural integrity. Here, single crystals of Zr2CuSb3, a potential candidate for the checkerboard lattice, were synthesized using the solution (self-flux) method, and their structure was confirmed via X-ray diffraction. Electrical transport measurements indicate metallic behavior with electron-dominated carriers. Angle-resolved photoemission spectroscopy reveals multiple electron pockets and significant kz broadening due to its large c-axis and low dispersion features in k z. Density functional theory calculations further disentangle the contributions from each high-symmetry plane, providing a comprehensive characterization of electronic behavior.
Authors
- Shane Smolenski (ORCID: https://orcid.org/0000-0002-7516-9316)
- Eli Rotenberg (ORCID: https://orcid.org/0000-0002-3979-8844)
- Demet Usanmaz (ORCID: https://orcid.org/0000-0001-8131-5589)
- Chris M. Jozwiak (ORCID: https://orcid.org/0000-0002-0980-3753)
- Aaron Bostwick (ORCID: https://orcid.org/0000-0002-9008-2980)
- Ruiqi Tang (ORCID: https://orcid.org/0000-0001-7759-0844)
- Anonymous
- Na Hyun Jo
- Soumya S. Bhat
- Carly Mistick
Institutions
- Lawrence Berkeley National Laboratory (US)
- University of Michigan (US)
- Kettering University (US)
Publication Details
- Journal
- Physical Review Materials
- Published
- 2026-01-02
- DOI
- https://doi.org/10.1103/qrll-lplv
- Primary Topic
- Rare-earth and actinide compounds
- Type
- article
- Field-Weighted Citation Impact
- 0.00